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Influence of high-fluence neutron and/or proton irradiation on the optical properties and microstructure of rutile
T. C. Lu; L. B. Lin; X. T. Zu; S. Zhu; L. M. Wang
2004
发表期刊Nuclear Instruments & Methods in Physics Research Section B-Beam Interactions with Materials and Atoms
ISSN0168-583X
卷号218页码:111-116
摘要Rutile (TiO2) single crystals of (1 1 0) or (0 0 1) orientation were irradiated by high fluence reactor neutrons with the fluence of 1 x 10(23) m(-2), by protons with the energy of 0.3-18 MeV and the fluence from 1 x 10(18) to 1.9 X 10(22) m(-2), respectively. UV-VIS-IR, LRS and HRTEM were used to analyze the optical properties and microstructure of samples. The UV-VIS-IR results showed that high-fluence neutron and proton irradiation induce similar variation of optical properties of samples, especially absorption plateau appear. LRS results showed that the relative intensity of common vibration modes is different for different plane, both high fluence neutron irradiation and proton irradiation induce similar variations of the frequency and intensity of Raman vibration modes in the same orientated samples, and proton irradiation also induces several new vibration modes appear. High fluence irradiation induced large defect clusters, i.e. stacking faults, which is demonstrated by HRTEM observation. In addition, the difference between neutron-induced irradiation effect and proton-induced irradiation effect has been also discussed. (C) 2004 Elsevier B.V. All rights reserved.
部门归属sichuan univ, dept phys, chengdu 610064, peoples r china. sichuan univ, key lab radiat phys & technol, minist educ, chengdu 610064, peoples r china. univ michigan, dept nucl engn & radiol sci, ann arbor, mi 48109 usa. chinese acad sci, int ctr mat phys, shenyang 110015, peoples r china.;lu, tc (reprint author), sichuan univ, dept phys, chengdu 610064, peoples r china;lutiecheng@sina.com
关键词Rutile Neutron Irradiation Proton Irradiation Optical Absorption Stacking Faults Tio2 Electrodes Ion Absorption Water
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WOS记录号WOS:000221561000017
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被引频次:21[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/35482
专题中国科学院金属研究所
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T. C. Lu,L. B. Lin,X. T. Zu,et al. Influence of high-fluence neutron and/or proton irradiation on the optical properties and microstructure of rutile[J]. Nuclear Instruments & Methods in Physics Research Section B-Beam Interactions with Materials and Atoms,2004,218:111-116.
APA T. C. Lu,L. B. Lin,X. T. Zu,S. Zhu,&L. M. Wang.(2004).Influence of high-fluence neutron and/or proton irradiation on the optical properties and microstructure of rutile.Nuclear Instruments & Methods in Physics Research Section B-Beam Interactions with Materials and Atoms,218,111-116.
MLA T. C. Lu,et al."Influence of high-fluence neutron and/or proton irradiation on the optical properties and microstructure of rutile".Nuclear Instruments & Methods in Physics Research Section B-Beam Interactions with Materials and Atoms 218(2004):111-116.
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