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Relaxation, nucleation, and glass transition in supercooled liquid Cu
H. Pang; Z. H. Jin; K. Lu
2003
Source PublicationPhysical Review B
ISSN1098-0121
Volume67Issue:9
AbstractUsing molecular-dynamics simulation with the embedded atom method, the dynamical properties of supercooled liquid Cu were studied by characterizing several time-correlation functions. With increasing undercooling of the liquid Cu below the melting point, self-diffusion slows down along with an increase in the structural relaxation time as compared with the normal liquid state. A massive structural rearrangement leading to incipient nucleation for crystallization occurs at a certain supercooling and time, underlying the existence of a transition in dynamical heterogeneities. Based on the temperature dependence of the characteristic relaxation times, a time-temperature-nucleation diagram has been constructed by which the relaxation, nucleation, and glass transition can be consistently correlated.
description.departmentchinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china. max planck inst met res, d-70569 stuttgart, germany.;pang, h (reprint author), chinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china
KeywordLennard-jones Mixture Mode-coupling Theory Crystal Nucleation Dynamics Metals Fragility Bcc
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WOS IDWOS:000182019300044
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Cited Times:66[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/35988
Collection中国科学院金属研究所
Recommended Citation
GB/T 7714
H. Pang,Z. H. Jin,K. Lu. Relaxation, nucleation, and glass transition in supercooled liquid Cu[J]. Physical Review B,2003,67(9).
APA H. Pang,Z. H. Jin,&K. Lu.(2003).Relaxation, nucleation, and glass transition in supercooled liquid Cu.Physical Review B,67(9).
MLA H. Pang,et al."Relaxation, nucleation, and glass transition in supercooled liquid Cu".Physical Review B 67.9(2003).
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