Relaxation, nucleation, and glass transition in supercooled liquid Cu | |
H. Pang; Z. H. Jin; K. Lu | |
2003 | |
Source Publication | Physical Review B
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ISSN | 1098-0121 |
Volume | 67Issue:9 |
Abstract | Using molecular-dynamics simulation with the embedded atom method, the dynamical properties of supercooled liquid Cu were studied by characterizing several time-correlation functions. With increasing undercooling of the liquid Cu below the melting point, self-diffusion slows down along with an increase in the structural relaxation time as compared with the normal liquid state. A massive structural rearrangement leading to incipient nucleation for crystallization occurs at a certain supercooling and time, underlying the existence of a transition in dynamical heterogeneities. Based on the temperature dependence of the characteristic relaxation times, a time-temperature-nucleation diagram has been constructed by which the relaxation, nucleation, and glass transition can be consistently correlated. |
description.department | chinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china. max planck inst met res, d-70569 stuttgart, germany.;pang, h (reprint author), chinese acad sci, inst met res, shenyang natl lab mat sci, shenyang 110016, peoples r china |
Keyword | Lennard-jones Mixture Mode-coupling Theory Crystal Nucleation Dynamics Metals Fragility Bcc |
URL | 查看原文 |
WOS ID | WOS:000182019300044 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/35988 |
Collection | 中国科学院金属研究所 |
Recommended Citation GB/T 7714 | H. Pang,Z. H. Jin,K. Lu. Relaxation, nucleation, and glass transition in supercooled liquid Cu[J]. Physical Review B,2003,67(9). |
APA | H. Pang,Z. H. Jin,&K. Lu.(2003).Relaxation, nucleation, and glass transition in supercooled liquid Cu.Physical Review B,67(9). |
MLA | H. Pang,et al."Relaxation, nucleation, and glass transition in supercooled liquid Cu".Physical Review B 67.9(2003). |
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