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PHASE-TRANSITION AND ELECTRON LOCALIZATION IN 1T-TAS2
S. Y. Dai; C. T. Yu; D. H. Li; Z. Y. Shen; S. Y. Fang
1995
发表期刊Physical Review B
ISSN0163-1829
卷号52期号:3页码:1578-1583
摘要The magnetic properties and phase transitions of 1T-TaS2 and 1T-Fe0.07Ta0.93S2 have been studied in the interval of 1.5-300 K and over the range of 100 Oe-60 kOe. Experimental results show that at high temperatures the compounds are in a diamagnetic state and the commensurate-charge-density-wave-triclinic-nearly-commensurate transition temperature of 1T-TaS2 decreases with increasing magnetic field. The amount of variation is a function of the magnetic field. At low temperatures both 1T-TaS2 and 1T-Fe0.07Ta0.93S2 are in a paramagnetic state owing to the localized moments that come from the single Anderson-Mott localization state. The curves of magnetization versus temperature do not follow the Curie law or Curie-Weiss law, but can be described fairly well as M = M(0) + gamma T--n. The fitting parameters of experimental curves show that a part of the neighboring moment appears as antiferromagnetic coupling due to exchange interaction between the moments. The magnetic-field dependence of magnetization exhibits a complicated feature at low temperature. It shows that the compounds may undergo a phase transition at the maximum value of magnetization and then they are probably in a mixed charge-density-wave-spin-density-wave (CDW-SDW) state or SDW state due to the coherent superposition of the antiferromagnetic coupling.
部门归属chinese acad sci, int ctr mat & phys, shenyang 110005, peoples r china. univ hunan, dept phys, changsha 410082, peoples r china.;dai, sy (reprint author), chinese acad sci, inst phys, beijing 100080, peoples r china, peoples r china
关键词Metal-insulator-transition Density-wave Domains High Magnetic-fields Charge-density Doped 1t-tas2 Coexistence Microscopy Systems Silicon 2h-tas2
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文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/38549
专题中国科学院金属研究所
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S. Y. Dai,C. T. Yu,D. H. Li,et al. PHASE-TRANSITION AND ELECTRON LOCALIZATION IN 1T-TAS2[J]. Physical Review B,1995,52(3):1578-1583.
APA S. Y. Dai,C. T. Yu,D. H. Li,Z. Y. Shen,&S. Y. Fang.(1995).PHASE-TRANSITION AND ELECTRON LOCALIZATION IN 1T-TAS2.Physical Review B,52(3),1578-1583.
MLA S. Y. Dai,et al."PHASE-TRANSITION AND ELECTRON LOCALIZATION IN 1T-TAS2".Physical Review B 52.3(1995):1578-1583.
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