MAGNETIC PHASE-TRANSITIONS, MAGNETOCRYSTALLINE ANISOTROPY, AND CRYSTAL-FIELD INTERACTIONS IN THE RFE11TI SERIES (WHERE R = Y, PR, ND, SM, GD, TB, DY, HO, ER, OR TM) | |
X. C. Kou; T. S. Zhao; R. Grossinger; H. R. Kirchmayr; X. Li; F. R. Deboer | |
1993 | |
发表期刊 | Physical Review B
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ISSN | 0163-1829 |
卷号 | 47期号:6页码:3231-3242 |
摘要 | A systematic investigation of the intrinsic magnetic properties of RFe11Ti compounds with R=Y, Pr, Nd, Sm, Gd, Th, Dy, Ho, Er, and Tm has been performed by means of ac susceptibility measurements, singular-point-detection techniques, and high-field magnetization measurements. Spin-reorientation transitions were observed in RFe11Ti with R=Nd (T(SR)=189 K), Tb (T(SR)=339 K), Dy (T(SR1)=214 K and T(SR2)=98 K), and Er (T(SR)=48 K). First-order magnetization processes of type I for R=Nd and Er and of type II for R=Ho and Tm were detected at low temperatures. The uniaxial magnetocrystalline anisotropy fields of the whole RFe11Ti series have been determined in a wide temperature interval from 4.2 K to the Curie temperatures. It is deduced that the ''anomalous increase'' in the magnetization curve of SmFe11Ti for the external field perpendicular to the c axis is not a first-order magnetization process, but a continuous rotation of the magnetic moment under the action of the external field. The observed magnetic phase transitions, the spin-reorientation transitions, and the first-order magnetization processes in the RFe11Ti compounds are well described in terms of a crystal-field description in which the rare-earth sublattice (R) and transition-metal sublattice (T) exchange interaction is included. A set of crystalline-electric-field parameters as well as the values for the R-T exchange field are deduced for the whole RFe11Ti series from fitting the experimentally obtained values of the anisotropy field, the critical field for the first-order magnetization process, and the spin-reorientation temperature with the calculations in the present systematic study. Magnetic anomalies are observed in the temperature dependence of the ac susceptibility of the RFe11Ti compounds with R=Nd, Sm, Er, and Tm. They are shown to be connected with domain-wall motion. |
部门归属 | acad sinica,inst met res,shenyang 110015,peoples r china. univ amsterdam,vanderwaals zeeman lab,1018 xe amsterdam,netherlands. jilin univ,dept phys,changchun 130023,peoples r china. vienna tech univ,inst exptl phys,a-1040 vienna,austria. |
关键词 | Spin-reorientation Single-crystal Intermetallic Compounds Fe Ti Nd2fe14b Susceptibility Exchange Systems Curve |
URL | 查看原文 |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/39050 |
专题 | 中国科学院金属研究所 |
推荐引用方式 GB/T 7714 | X. C. Kou,T. S. Zhao,R. Grossinger,et al. MAGNETIC PHASE-TRANSITIONS, MAGNETOCRYSTALLINE ANISOTROPY, AND CRYSTAL-FIELD INTERACTIONS IN THE RFE11TI SERIES (WHERE R = Y, PR, ND, SM, GD, TB, DY, HO, ER, OR TM)[J]. Physical Review B,1993,47(6):3231-3242. |
APA | X. C. Kou,T. S. Zhao,R. Grossinger,H. R. Kirchmayr,X. Li,&F. R. Deboer.(1993).MAGNETIC PHASE-TRANSITIONS, MAGNETOCRYSTALLINE ANISOTROPY, AND CRYSTAL-FIELD INTERACTIONS IN THE RFE11TI SERIES (WHERE R = Y, PR, ND, SM, GD, TB, DY, HO, ER, OR TM).Physical Review B,47(6),3231-3242. |
MLA | X. C. Kou,et al."MAGNETIC PHASE-TRANSITIONS, MAGNETOCRYSTALLINE ANISOTROPY, AND CRYSTAL-FIELD INTERACTIONS IN THE RFE11TI SERIES (WHERE R = Y, PR, ND, SM, GD, TB, DY, HO, ER, OR TM)".Physical Review B 47.6(1993):3231-3242. |
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