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Development of Cu foam-based Ni catalyst for solar thermal reforming of methane with carbon dioxide
Qi, Jianzhong; Sun, Yanping; Xie, Zongli; Collins, Mike; Du, Hao; Xiong, Tianying; Yanping.Sun@csiro.au
2015
Source PublicationJOURNAL OF ENERGY CHEMISTRY
ISSN2095-4956
Volume24Issue:6Pages:786-793
AbstractUsing solar energy to produce syngas via the endothermic reforming of methane has been extensively investigated at the laboratory- and pilot plant-scales as a promising method of storing solar energy. One of the challenges to scaling up this process in a tubular reformer is to improve the reactor's performance, which is limited by mass and heat transfer issues. High thermal conductivity Cu foam was therefore used as a substrate to improve the catalyst's thermal conductivity during solar reforming. We also developed a method to coat the foam with the catalytically active component NiMg3AlOx. The Cu foam-based NiMg3AlOx performs better than catalysts supported on SiSiC foam, which is currently used as a substrate for solar-reforming catalysts, at high gas hourly space velocity (>= 400,000 mL/(g.h)) or at low reaction temperatures (<= 720 degrees C). The presence of a gamma-Al2O3 intermediate layer improves the adhesion between the catalyst and substrate as well as the catalytic activity. (C) 2015 Science Press and Dalian Institute of Chemical Physics. All rights reserved.
description.department[qi, jianzhong ; du, hao ; xiong, tianying] chinese acad sci, inst met res, shenyang 110016, liaoning, peoples r china ; [sun, yanping ; collins, mike] csiro energy flagship, newcastle, nsw 2300, australia ; [xie, zongli] csiro mfg flagship, clayton, vic 3169, australia
KeywordCu Foam-based Ni Catalyst Monolithic Catalyst Solar Thermal Reforming Of Methane
Funding OrganizationCSIRO Energy Flagship; Chinese Scholarship Council
Indexed Bysci
Language英语
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/74717
Collection中国科学院金属研究所
Corresponding AuthorYanping.Sun@csiro.au
Recommended Citation
GB/T 7714
Qi, Jianzhong,Sun, Yanping,Xie, Zongli,et al. Development of Cu foam-based Ni catalyst for solar thermal reforming of methane with carbon dioxide[J]. JOURNAL OF ENERGY CHEMISTRY,2015,24(6):786-793.
APA Qi, Jianzhong.,Sun, Yanping.,Xie, Zongli.,Collins, Mike.,Du, Hao.,...&Yanping.Sun@csiro.au.(2015).Development of Cu foam-based Ni catalyst for solar thermal reforming of methane with carbon dioxide.JOURNAL OF ENERGY CHEMISTRY,24(6),786-793.
MLA Qi, Jianzhong,et al."Development of Cu foam-based Ni catalyst for solar thermal reforming of methane with carbon dioxide".JOURNAL OF ENERGY CHEMISTRY 24.6(2015):786-793.
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