IMR OpenIR
Vapor-Dissociation-Solid Growth of Three-Dimensional Graphite like Capsules with Delicate Morphology and Atomic-level Thickness Control
Jian, X; Chen, GZ; Liu, HY; Mahmood, N; Zhu, SB; Yin, LJ; Tang, H; Lv, WQ; He, WD; Zhang, KHL; Zeng, Q; Li, BH; Li, XS; Zhang, WL; Wang, XL; He, WD (reprint author), Univ Elect Sci & Technol China, Sch Energy Sci & Engn, Ctr Micronano Funct Mat & Devices, Chengdu 611731, Peoples R China.; Wang, XL (reprint author), Univ Wollongong, Australian Inst Innovat Mat, Inst Superconducting & Elect Mat, North Wollongong 2500, Australia.; Zeng, Q (reprint author), China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Peoples R China.; Zhang, WL (reprint author), Univ Elect Sci & Technol China, Inst Microelect & Solid State Elect, State key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China.
2016-09-01
发表期刊CRYSTAL GROWTH & DESIGN
ISSN1528-7483
卷号16期号:9页码:5040-5048
摘要Two-dimensional graphene is easy to aggregate and hard to transfer because of the van der Waals forces between graphene layers. The three-dimensional (3D) graphite-like capsules (GCs) disperse well and exhibit robust structural stability and have a potential for promising applications in energy storage, drug delivery, catalyst substrate, etc. Here, we develop a catalytic chemical vapor deposition route for the synthesis of 3D GCs with unprecedented thickness and morphology control. The theoretical results indicate that the strong chemisorption and charge transfer between ZnO and acetylene allow the layer-by-layer formation of GCs that is later confirmed by the experimental data. The 3D GCs are synthesized with thickness control from three atomic layers to similar to 300 atomic layers over various oxides with predesigned shapes of microscale tetrapods, nanospheres, nanorods, nanocubes, etc. In particular, the formation mechanism of GCs is investigated using the ZnO surface as a catalyst through systematically experimental approaches. In addition to the high-quality of 3D GCs, this approach provides an unprecedented facile methodological control of coating/functionalizing carbon over various oxides including ZnO, TiO2, SnO2, BaFe12O19, etc.
部门归属[jian, xian ; chen, guozhang ; yin, liangjun ; tang, hui ; lv, weiqiang ; he, weidong ; li, baihai] univ elect sci & technol china, sch energy sci & engn, ctr micronano funct mat & devices, chengdu 611731, peoples r china ; [jian, xian ; mahmood, nasir ; wang, xiaolin] univ wollongong, australian inst innovat mat, inst superconducting & elect mat, north wollongong 2500, australia ; [liu, hongyang] chinese acad sci, shenyang natl lab mat sci, inst met res, shenyang 110016, peoples r china ; [zhu, shibu] xian aerosp composites res inst, xian 710025, peoples r china ; [zhang, kelvin h. l.] univ cambridge, dept mat sci & met, 27 charles babbage rd, cambridge cb3 0fs, england ; [zeng, qun] china acad engn phys, inst chem mat, mianyang 621900, peoples r china ; [li, xuesong ; zhang, wanli] univ elect sci & technol china, inst microelect & solid state elect, state key lab elect thin films & integrated devic, chengdu 610054, peoples r china
学科领域Chemistry, Multidisciplinary ; Crystallography ; Materials Science, Multidisciplinary
资助者National Natural Science Foundation of China [51402040]; China Postdoctoral Science Foundation [2015M582539]; Science and Technology Support Program of Sichuan Province [2016RZ0054]; Open Foundation of State Key Laboratory of Electronic Thin Films and Integrated Devices [KFJJ201411]; National Hi-Tech Research and Development Program (863 Program) of China [2015AA034202]; Automotive CRC, Common Wealth of Australia [1-108]
收录类别sci
语种英语
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/76285
专题中国科学院金属研究所
通讯作者He, WD (reprint author), Univ Elect Sci & Technol China, Sch Energy Sci & Engn, Ctr Micronano Funct Mat & Devices, Chengdu 611731, Peoples R China.; Wang, XL (reprint author), Univ Wollongong, Australian Inst Innovat Mat, Inst Superconducting & Elect Mat, North Wollongong 2500, Australia.; Zeng, Q (reprint author), China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Peoples R China.; Zhang, WL (reprint author), Univ Elect Sci & Technol China, Inst Microelect & Solid State Elect, State key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China.
推荐引用方式
GB/T 7714
Jian, X,Chen, GZ,Liu, HY,et al. Vapor-Dissociation-Solid Growth of Three-Dimensional Graphite like Capsules with Delicate Morphology and Atomic-level Thickness Control[J]. CRYSTAL GROWTH & DESIGN,2016,16(9):5040-5048.
APA Jian, X.,Chen, GZ.,Liu, HY.,Mahmood, N.,Zhu, SB.,...&Zhang, WL .(2016).Vapor-Dissociation-Solid Growth of Three-Dimensional Graphite like Capsules with Delicate Morphology and Atomic-level Thickness Control.CRYSTAL GROWTH & DESIGN,16(9),5040-5048.
MLA Jian, X,et al."Vapor-Dissociation-Solid Growth of Three-Dimensional Graphite like Capsules with Delicate Morphology and Atomic-level Thickness Control".CRYSTAL GROWTH & DESIGN 16.9(2016):5040-5048.
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