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Interfacial Fe 5 C 2 -Cu catalysts toward low-pressure syngas conversion to long-chain alcohols
Yinwen Li; Wa Gao; Mi Peng; Junbo Zhang; Jialve Sun; Yao Xu; Song Hong; Xi Liu; Xingwu Liu; Min Wei; Bingsen Zhang; Ding Ma
2020
Source Publicationnaturecommunications
ISSN2041-1723
Volume11Issue:1Pages:1-8
AbstractLong-chain alcohols synthesis (LAS, C 5+ OH) from syngas provides a promising route for the conversion of coal 5 C 2 -Cu interfacial catalyst derived from Cu 4 Fe 1 Mg 4 -layered double hydroxide (Cu 4 Fe 1 Mg 4 -LDH) precursor, i.e ., Fe 5 C 2 clusters (~2?nm) are immobilized onto the surface of Cu nanoparticles (~25?nm). The interfacial catalyst exhibits a CO conversion of 53.2%, a selectivity of 14.8?mol% and a space time yield of 0.101?g g cat ?1 h ?1 for long-chain alcohols, with a surprisingly benign reaction pressure of 1?MPa. This catalytic performance, to the best of our knowledge, is comparable to the optimal level of Cu-Fe catalysts operated at much higher pressure (normally above 3?MPa).
DOI10.1038/s41467-019-13691-4
Language英语
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/80694
Collection中国科学院金属研究所
Affiliation1.Beijing University of Chemical Technology
2.College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
3.State Key Laboratory of Coal Conversion, Institute of Coal Chemistry Chinese Academy of Sciences Taiyuan
4.Synfuels China Beijing
5.Institute of Metal Research, Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Yinwen Li,Wa Gao,Mi Peng,et al. Interfacial Fe 5 C 2 -Cu catalysts toward low-pressure syngas conversion to long-chain alcohols[J]. naturecommunications,2020,11(1):1-8.
APA Yinwen Li.,Wa Gao.,Mi Peng.,Junbo Zhang.,Jialve Sun.,...&Ding Ma.(2020).Interfacial Fe 5 C 2 -Cu catalysts toward low-pressure syngas conversion to long-chain alcohols.naturecommunications,11(1),1-8.
MLA Yinwen Li,et al."Interfacial Fe 5 C 2 -Cu catalysts toward low-pressure syngas conversion to long-chain alcohols".naturecommunications 11.1(2020):1-8.
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