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The synthesis of nitrogen/sulfur co-doped TiO2 nanocrystals with a high specific surface area and a high percentage of {001} facets and their enhanced visible-light photocatalytic performance
Shi,Wenjing1; Yang,Weiyi1; Li,Qi1; Gao,Shian1; Shang,Panju1; Shang,Jian Ku1,2
通讯作者Li,Qi(qili@imr.ac.cn)
2012-10-24
发表期刊Nanoscale Research Letters
ISSN1556-276X
卷号7期号:1
摘要AbstractNitrogen/sulfur co-doped anatase TiO2 nanocrystals with a high specific surface area and a high percentage of {001} facets were synthesized by a solvent-thermal process followed by the calcination with thiourea at an optimum heat treatment temperature. Under current experimental conditions, the optimum heat treatment temperature was found at 300°C, which successfully introduced nitrogen and sulfur dopants into the anatase lattice to replace a small portion of oxygen atoms while preserving the geometry of these anatase TiO2 nanocrystals to maintain a high percentage of {001} facets. These nitrogen/sulfur co-doped anatase TiO2 nanocrystals demonstrated a largely enhanced light absorption in the whole visible-light range and exhibited much higher photocatalytic performance than both P25 TiO2 nanoparticles and anatase TiO2 nanocrystals with a high percentage of {001} facets under visible-light illumination.
关键词TiO2 nanocrystals Highly active {001} facets Nitrogen/sulfur co-doped Visible-light photocatalytic performance
DOI10.1186/1556-276X-7-590
语种英语
WOS记录号BMC:10.1186/1556-276X-7-590
出版者Springer New York
引用统计
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/80781
通讯作者Li,Qi
作者单位1.Chinese Academy of Sciences; Materials Center for Water Purification, Shenyang National Laboratory for Materials Science, Institute of Metal Research
2.University of Illinois at Urbana-Champaign; Department of Materials Science and Engineering
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Shi,Wenjing,Yang,Weiyi,Li,Qi,et al. The synthesis of nitrogen/sulfur co-doped TiO2 nanocrystals with a high specific surface area and a high percentage of {001} facets and their enhanced visible-light photocatalytic performance[J]. Nanoscale Research Letters,2012,7(1).
APA Shi,Wenjing,Yang,Weiyi,Li,Qi,Gao,Shian,Shang,Panju,&Shang,Jian Ku.(2012).The synthesis of nitrogen/sulfur co-doped TiO2 nanocrystals with a high specific surface area and a high percentage of {001} facets and their enhanced visible-light photocatalytic performance.Nanoscale Research Letters,7(1).
MLA Shi,Wenjing,et al."The synthesis of nitrogen/sulfur co-doped TiO2 nanocrystals with a high specific surface area and a high percentage of {001} facets and their enhanced visible-light photocatalytic performance".Nanoscale Research Letters 7.1(2012).
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