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Fabrication of mesoporous MOF nanosheets via surfactant-template method for C-S coupling reactions
Wang, Sha; Wang, Tieqiang; Zheng, Huayu; Fan, Fuqiang; Gu, Zhida; He, Wenxiu; Zhang, Bing; Shao, Lei; Chen, Huan; Li, Yunong; Zhang, Xuemin; Zhang, Liying; Fu, Yu; Qi, Wei
2020-08-15
Source PublicationMICROPOROUS AND MESOPOROUS MATERIALS
Volume303
AbstractPore size enlargement plays a vital role in the catalytic applications of metal-organic frameworks (MOFs). There is still a big challenge in achieving two-dimension (2D) ultrathin MOF nanosheets with controllable meso-pores, although it has huge demanding. In this work, various kinds of mesoporous MOF nanosheets with uniform mesopore channels and crystallized microporous frameworks were constructed using surfactants (cetyltrimethyl ammonium bromide, CTAB) as sacrificial templates. CTAB was firstly introduced into MOF nanosheet structure during the formation of MOF nanosheets, and mesopores could be produced by removing CTAB from MOF nanosheets. Remarkably, the integration of ultrathin nanosheets and mesoporous property enables mesoporous CuBDC nanosheets enhanced catalytic activity for C-S cross-coupling reaction, providing a new concept and feasible strategy for highly efficient mesoporous MOF catalyst synthesis.
DOI10.1016/j.micromeso.2020.110254
WOS IDWOS:000535938200015
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Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/82625
Collection中国科学院金属研究所
Recommended Citation
GB/T 7714
Wang, Sha,Wang, Tieqiang,Zheng, Huayu,et al. Fabrication of mesoporous MOF nanosheets via surfactant-template method for C-S coupling reactions[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2020,303.
APA Wang, Sha.,Wang, Tieqiang.,Zheng, Huayu.,Fan, Fuqiang.,Gu, Zhida.,...&Qi, Wei.(2020).Fabrication of mesoporous MOF nanosheets via surfactant-template method for C-S coupling reactions.MICROPOROUS AND MESOPOROUS MATERIALS,303.
MLA Wang, Sha,et al."Fabrication of mesoporous MOF nanosheets via surfactant-template method for C-S coupling reactions".MICROPOROUS AND MESOPOROUS MATERIALS 303(2020).
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