Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O

doi:10.1016/j.jmmm.2008.01.033

IMR OpenIR

	Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O
	Li, Z. B.1; Yao, K. L.2,3; Liu, Z. Li 2
通讯作者	Li, Z. B.(zongbaoli1982@gmail.com)
	2008-06-01
发表期刊	JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
ISSN	0304-8853
卷号	320 期号:11 页码:1759-1764
摘要	The magnetic and thermodynamic properties of the spin-1 tetrahedral "Ni-4'' model have been investigated in terms of the Heisenberg model by algebraic method. It is shown that the Heisenberg model provides an adequate description of the magnetization at low temperatures. The temperature dependence of the specific heat of this model in the vicinity of the midpoint at the rising magnetization M shows remarkable double-peak structure due to the ferromagnetic gapless and anti-ferromagnetic gap excitation of the spin system. The magnetization curve has four clear plateaus, and the susceptibilities exhibit typical anti-ferromagnetic feature, which is well consistent with experimental findings. In particular, the critical magnetic field values H-1 = 5.40 T, H-2 10.69 T, H-3 16.05T and H-4 28.06 T corresponding to the magnetization plateaus are in quantitative agreement with the experimental observations and the former theoretical calculation. (C) 2008 Elsevier B.V. All rights reserved.
关键词	high-pulsed magnetic field Heisenberg model magnetization susceptibility
DOI	10.1016/j.jmmm.2008.01.033
收录类别	SCI
语种	英语
WOS研究方向	Materials Science ; Physics
WOS类目	Materials Science, Multidisciplinary ; Physics, Condensed Matter
WOS记录号	WOS:000255512200006
出版者	ELSEVIER SCIENCE BV
引用统计	被引频次：7[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/93929
专题	中国科学院金属研究所
通讯作者	Li, Z. B.
作者单位	1.Tongren Univ, Dept Phys, Guizhou 554300, Peoples R China 2.Huazhong Univ Sci & Technol, Dept Phys, Wuhan 430074, Peoples R China 3.Chinese Acad Sci, Int Ctr Mat Phys, Shenyang 110016, Peoples R China
推荐引用方式 GB/T 7714	Li, Z. B.,Yao, K. L.,Liu, Z. Li. Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O[J]. JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS,2008,320(11):1759-1764.
APA	Li, Z. B.,Yao, K. L.,&Liu, Z. Li.(2008).Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O.JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS,320(11),1759-1764.
MLA	Li, Z. B.,et al."Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O".JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 320.11(2008):1759-1764.