Highly efficient H-2 evolution over ZnO-ZnS-CdS heterostructures from an aqueous solution containing SO32- and S2- ions | |
Wang, Xuewen3; Liu, Gang3; Chen, Zhi-Gang3; Li, Feng3; Lu, Gao Qing1,2; Cheng, Hui-Ming3 | |
通讯作者 | Lu, Gao Qing(maxlu@uq.edu.au) |
2010 | |
发表期刊 | JOURNAL OF MATERIALS RESEARCH
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ISSN | 0884-2914 |
卷号 | 25期号:1页码:39-44 |
摘要 | ZnO-ZnS-CdS heterostructure photocatalysts for water splitting were designed and prepared by a wet chemistry method. It was found that ZnO-ZnS-CdS heterostructures are highly active photocatalysts for H-2 evolution under simulated solar light irradiation in an aqueous solution containing SO32- and S2- ions as sacrificial reagents. H-2 evolution with (ZnO)(2)-(ZnS)(1)-(CdS)(1) heterostructure reaches up to 2790 mu mol h(-1) g(-1). The photoexcited electrons in the ZnO-ZnS-CdS heterostructures have a much longer lifetime (>225 ns) than that of the sole ZnO, ZnS, and CdS (<65 ns). The favorable interface processes of the heterostructures make a significant contribution to high photocatalytic H-2 evolution rate. |
资助者 | Chinese Academy of Sciences ; Ministry of Science and Technology China ; Australian Research Council |
DOI | 10.1557/JMR.2010.0018 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | Chinese Academy of Sciences[GJHZ200815] ; Ministry of Science and Technology China[2009CB220001] ; Australian Research Council |
WOS研究方向 | Materials Science |
WOS类目 | Materials Science, Multidisciplinary |
WOS记录号 | WOS:000273858900006 |
出版者 | CAMBRIDGE UNIV PRESS |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/99852 |
专题 | 中国科学院金属研究所 |
通讯作者 | Lu, Gao Qing |
作者单位 | 1.Univ Queensland, Sch Engn, ARC Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia 2.Univ Queensland, Australian Inst Bioengn & Nanotechnol, Brisbane, Qld 4072, Australia 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Xuewen,Liu, Gang,Chen, Zhi-Gang,et al. Highly efficient H-2 evolution over ZnO-ZnS-CdS heterostructures from an aqueous solution containing SO32- and S2- ions[J]. JOURNAL OF MATERIALS RESEARCH,2010,25(1):39-44. |
APA | Wang, Xuewen,Liu, Gang,Chen, Zhi-Gang,Li, Feng,Lu, Gao Qing,&Cheng, Hui-Ming.(2010).Highly efficient H-2 evolution over ZnO-ZnS-CdS heterostructures from an aqueous solution containing SO32- and S2- ions.JOURNAL OF MATERIALS RESEARCH,25(1),39-44. |
MLA | Wang, Xuewen,et al."Highly efficient H-2 evolution over ZnO-ZnS-CdS heterostructures from an aqueous solution containing SO32- and S2- ions".JOURNAL OF MATERIALS RESEARCH 25.1(2010):39-44. |
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