The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study | |
Ma, Yunhai1; Cai, Dali1; Li, Yiru1; Wang, Ning1; Muhammad, Usman1; Carlsson, Anna2; Tang, Dong2; Qian, Weizhong1; Wang, Yao1; Su, Dangsheng3; Wei, Fei1 | |
Corresponding Author | Qian, Weizhong(qianwz@mail.tsinghua.edu.cn) ; Wei, Fei(wf-dce@tsinghua.edu.cn) |
2016 | |
Source Publication | RSC ADVANCES
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ISSN | 2046-2069 |
Volume | 6Issue:78Pages:74797-74801 |
Abstract | Here we report the direct atomic scale observation of ZSM-5 pores and the influence of extra-framework Al on methanol to aromatic (MTA). We synthesized a nano sized ZSM-5 catalyst with a short b-axis, and fully opened straight channels. A 98% ultrahigh aromatic selectivity, more than 300 hours long life time and high anti-hydrothermal ability can be achieved in the MTA process. |
Funding Organization | NSFC program ; CNPC Innovation Foundation |
DOI | 10.1039/c6ra19073a |
Indexed By | SCI |
Language | 英语 |
Funding Project | NSFC program[21376135] ; NSFC program[91434122] ; NSFC program[51236004] ; CNPC Innovation Foundation[2014D-5006-0506] |
WOS Research Area | Chemistry |
WOS Subject | Chemistry, Multidisciplinary |
WOS ID | WOS:000381513600100 |
Publisher | ROYAL SOC CHEMISTRY |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/122783 |
Collection | 中国科学院金属研究所 |
Corresponding Author | Qian, Weizhong; Wei, Fei |
Affiliation | 1.Tsinghua Univ, Dept Chem Engn, Beijing 100084, Peoples R China 2.FEI NanoPort Europe, NL-5611 GG Eindhoven, Netherlands 3.Chinese Acad Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110006, Peoples R China |
Recommended Citation GB/T 7714 | Ma, Yunhai,Cai, Dali,Li, Yiru,et al. The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study[J]. RSC ADVANCES,2016,6(78):74797-74801. |
APA | Ma, Yunhai.,Cai, Dali.,Li, Yiru.,Wang, Ning.,Muhammad, Usman.,...&Wei, Fei.(2016).The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study.RSC ADVANCES,6(78),74797-74801. |
MLA | Ma, Yunhai,et al."The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study".RSC ADVANCES 6.78(2016):74797-74801. |
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