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The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study
Ma, Yunhai1; Cai, Dali1; Li, Yiru1; Wang, Ning1; Muhammad, Usman1; Carlsson, Anna2; Tang, Dong2; Qian, Weizhong1; Wang, Yao1; Su, Dangsheng3; Wei, Fei1
通讯作者Qian, Weizhong(qianwz@mail.tsinghua.edu.cn) ; Wei, Fei(wf-dce@tsinghua.edu.cn)
2016
发表期刊RSC ADVANCES
ISSN2046-2069
卷号6期号:78页码:74797-74801
摘要Here we report the direct atomic scale observation of ZSM-5 pores and the influence of extra-framework Al on methanol to aromatic (MTA). We synthesized a nano sized ZSM-5 catalyst with a short b-axis, and fully opened straight channels. A 98% ultrahigh aromatic selectivity, more than 300 hours long life time and high anti-hydrothermal ability can be achieved in the MTA process.
资助者NSFC program ; CNPC Innovation Foundation
DOI10.1039/c6ra19073a
收录类别SCI
语种英语
资助项目NSFC program[21376135] ; NSFC program[91434122] ; NSFC program[51236004] ; CNPC Innovation Foundation[2014D-5006-0506]
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000381513600100
出版者ROYAL SOC CHEMISTRY
引用统计
被引频次:54[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/122783
专题中国科学院金属研究所
通讯作者Qian, Weizhong; Wei, Fei
作者单位1.Tsinghua Univ, Dept Chem Engn, Beijing 100084, Peoples R China
2.FEI NanoPort Europe, NL-5611 GG Eindhoven, Netherlands
3.Chinese Acad Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110006, Peoples R China
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Ma, Yunhai,Cai, Dali,Li, Yiru,et al. The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study[J]. RSC ADVANCES,2016,6(78):74797-74801.
APA Ma, Yunhai.,Cai, Dali.,Li, Yiru.,Wang, Ning.,Muhammad, Usman.,...&Wei, Fei.(2016).The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study.RSC ADVANCES,6(78),74797-74801.
MLA Ma, Yunhai,et al."The influence of straight pore blockage on the selectivity of methanol to aromatics in nanosized Zn/ZSM-5: an atomic Cs-corrected STEM analysis study".RSC ADVANCES 6.78(2016):74797-74801.
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