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Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints
Xie, Bijun1,2; Sun, Mingyue1,3; Xu, Bin1,3; Wang, Chunyang1,2; Li, Dianzhong1; Li, Yiyi1
Corresponding AuthorSun, Mingyue(mysun@imr.ac.cn)
2018-11-05
Source PublicationMATERIALS & DESIGN
ISSN0264-1275
Volume157Pages:437-446
AbstractThe mechanical properties of solid state bonding joints have always been greatly deteriorated due to surface oxide scales. Here, we report a method to completely heal solid state bonding joints with recovered mechanical properties by hot compression bonding and post-holding treatment. Using scanning electron microscopy and transmission electron microscopy, we discovered that the recovery of mechanical properties of the bonding joint is attributed to the dissolution and evolution of the interfacial oxides. While holding the joint at 1200 degrees C, the interfacial oxides (MnCr2O4) gradually decomposed. With the decomposed oxygen ions diffusing toward the matrix, oxide particles precipitated around both sides of the interface, forming the particle precipitation zone (PPZ). As the holding time increased, the width of the PPZ increased and the oxide precipitates in the PPZ transformed from MnCrxAl2-xO4 to MnxAl3-xO4 and finally to gamma-Al2O3, depending on the local oxygen activity. After holding for 24 h, the interfacial oxides completely decomposed and only a few nano-scale gamma-Al2O3 oxide precipitates remained dispersed far away from the bonding interface, leading to the recovery of the mechanical properties of the bonding joints. This recovery mechanism may be of great importance to the design and manufacture of high-quality heavy bonding joints. (C) 2018 Elsevier Ltd. All rights reserved.
KeywordHot compression bonding Interfacial oxides Mechanical properties TEM Interface healing
Funding OrganizationNational Key Research and Development program ; National Natural Science Foundation of China ; key Program of the Chinese Academy of Sciences
DOI10.1016/j.matdes.2018.08.003
Indexed BySCI
Language英语
Funding ProjectNational Key Research and Development program[2016YFB0300401] ; National Natural Science Foundation of China[U1508215] ; National Natural Science Foundation of China[51774265] ; key Program of the Chinese Academy of Sciences[ZDRW-CN-2017-1]
WOS Research AreaMaterials Science
WOS SubjectMaterials Science, Multidisciplinary
WOS IDWOS:000443826600041
PublisherELSEVIER SCI LTD
Citation statistics
Cited Times:49[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/129373
Collection中国科学院金属研究所
Corresponding AuthorSun, Mingyue
Affiliation1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Key Lab Nucl Mat & Safety Assessment, Shenyang 110016, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Xie, Bijun,Sun, Mingyue,Xu, Bin,et al. Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints[J]. MATERIALS & DESIGN,2018,157:437-446.
APA Xie, Bijun,Sun, Mingyue,Xu, Bin,Wang, Chunyang,Li, Dianzhong,&Li, Yiyi.(2018).Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints.MATERIALS & DESIGN,157,437-446.
MLA Xie, Bijun,et al."Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints".MATERIALS & DESIGN 157(2018):437-446.
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