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Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints
Xie, Bijun1,2; Sun, Mingyue1,3; Xu, Bin1,3; Wang, Chunyang1,2; Li, Dianzhong1; Li, Yiyi1
通讯作者Sun, Mingyue(mysun@imr.ac.cn)
2018-11-05
发表期刊MATERIALS & DESIGN
ISSN0264-1275
卷号157页码:437-446
摘要The mechanical properties of solid state bonding joints have always been greatly deteriorated due to surface oxide scales. Here, we report a method to completely heal solid state bonding joints with recovered mechanical properties by hot compression bonding and post-holding treatment. Using scanning electron microscopy and transmission electron microscopy, we discovered that the recovery of mechanical properties of the bonding joint is attributed to the dissolution and evolution of the interfacial oxides. While holding the joint at 1200 degrees C, the interfacial oxides (MnCr2O4) gradually decomposed. With the decomposed oxygen ions diffusing toward the matrix, oxide particles precipitated around both sides of the interface, forming the particle precipitation zone (PPZ). As the holding time increased, the width of the PPZ increased and the oxide precipitates in the PPZ transformed from MnCrxAl2-xO4 to MnxAl3-xO4 and finally to gamma-Al2O3, depending on the local oxygen activity. After holding for 24 h, the interfacial oxides completely decomposed and only a few nano-scale gamma-Al2O3 oxide precipitates remained dispersed far away from the bonding interface, leading to the recovery of the mechanical properties of the bonding joints. This recovery mechanism may be of great importance to the design and manufacture of high-quality heavy bonding joints. (C) 2018 Elsevier Ltd. All rights reserved.
关键词Hot compression bonding Interfacial oxides Mechanical properties TEM Interface healing
资助者National Key Research and Development program ; National Natural Science Foundation of China ; key Program of the Chinese Academy of Sciences
DOI10.1016/j.matdes.2018.08.003
收录类别SCI
语种英语
资助项目National Key Research and Development program[2016YFB0300401] ; National Natural Science Foundation of China[U1508215] ; National Natural Science Foundation of China[51774265] ; key Program of the Chinese Academy of Sciences[ZDRW-CN-2017-1]
WOS研究方向Materials Science
WOS类目Materials Science, Multidisciplinary
WOS记录号WOS:000443826600041
出版者ELSEVIER SCI LTD
引用统计
被引频次:76[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/129373
专题中国科学院金属研究所
通讯作者Sun, Mingyue
作者单位1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Key Lab Nucl Mat & Safety Assessment, Shenyang 110016, Liaoning, Peoples R China
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GB/T 7714
Xie, Bijun,Sun, Mingyue,Xu, Bin,et al. Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints[J]. MATERIALS & DESIGN,2018,157:437-446.
APA Xie, Bijun,Sun, Mingyue,Xu, Bin,Wang, Chunyang,Li, Dianzhong,&Li, Yiyi.(2018).Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints.MATERIALS & DESIGN,157,437-446.
MLA Xie, Bijun,et al."Dissolution and evolution of interfacial oxides improving the mechanical properties of solid state bonding joints".MATERIALS & DESIGN 157(2018):437-446.
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