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Structured ZSM-5 coated SiC foam catalysts for process intensification in catalytic cracking of n-hexane\
Jiao, Yilai1,2; Ou, Xiaoxia2; Zhang, Jinsong1; Fan, Xiaolei2
Corresponding AuthorJiao, Yilai(yljiao@imr.ac.cn) ; Fan, Xiaolei(Xiaolei.fan@manchester.ac.uk)
2019-02-01
Source PublicationREACTION CHEMISTRY & ENGINEERING
ISSN2058-9883
Volume4Issue:2Pages:427-435
AbstractStructured foam catalysts are materials that address the mass and heat transfer limitations in catalytic processes. In this work, ZSM-5 coated silicon carbide (SiC) foams were prepared by a dispersion-based method, resulting in a thin and uniform zeolite layer on the foam support (i.e. ZSM-5/SiC foam catalysts). A comparative study of catalytic cracking of n-hexane was studied over ZSM-5/SiC foam and ZSM-5 pellet catalysts at space velocities of 4-40 h(-1), showing the improved n-hexane conversion, total selectivity to C-2-C-4 olefins and anti-deactivation performance, especially at the relatively high space velocities (>10 h(-1)), achieved by the ZSM-5/SiC foam catalysts. The yield of light olefins obtained by the ZSM-5/SiC foam catalyst (with 45 ppi cell density) was almost five times higher than the yield obtained by the conventional ZSM-5 pellets. A detailed analysis revealed that the specific surface area of SiC foams has a significant effect on the coating quality, and hence, the catalytic performance in the cracking reaction.
Funding OrganizationEngineering and Physical Sciences Research Council ; Liaoning Provincial Natural Science Foundation of China ; National 863 Program of China ; China Scholarship Council (CSC)
DOI10.1039/c8re00215k
Indexed BySCI
Language英语
Funding ProjectEngineering and Physical Sciences Research Council[EP/R000670/1] ; Liaoning Provincial Natural Science Foundation of China[20180510012] ; National 863 Program of China[2012AA030304] ; China Scholarship Council (CSC)[201604910181]
WOS Research AreaChemistry ; Engineering
WOS SubjectChemistry, Multidisciplinary ; Engineering, Chemical
WOS IDWOS:000459587000022
PublisherROYAL SOC CHEMISTRY
Citation statistics
Cited Times:14[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/132082
Collection中国科学院金属研究所
Corresponding AuthorJiao, Yilai; Fan, Xiaolei
Affiliation1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
2.Univ Manchester, Sch Chem Engn & Analyt Sci, Oxford Rd, Manchester M13 9PL, Lancs, England
Recommended Citation
GB/T 7714
Jiao, Yilai,Ou, Xiaoxia,Zhang, Jinsong,et al. Structured ZSM-5 coated SiC foam catalysts for process intensification in catalytic cracking of n-hexane\[J]. REACTION CHEMISTRY & ENGINEERING,2019,4(2):427-435.
APA Jiao, Yilai,Ou, Xiaoxia,Zhang, Jinsong,&Fan, Xiaolei.(2019).Structured ZSM-5 coated SiC foam catalysts for process intensification in catalytic cracking of n-hexane\.REACTION CHEMISTRY & ENGINEERING,4(2),427-435.
MLA Jiao, Yilai,et al."Structured ZSM-5 coated SiC foam catalysts for process intensification in catalytic cracking of n-hexane\".REACTION CHEMISTRY & ENGINEERING 4.2(2019):427-435.
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