Synthesis and photo-catalytic activity of porous g-C3N4: Promotion effect of nitrogen vacancy in H-2 evolution and pollutant degradation reactions | |
Liang, Lei1; Shi, Lei1; Wang, Fangxiao2; Yao, Lizhu1; Zhang, Ying1; Qi, Wei3 | |
Corresponding Author | Shi, Lei(shilei_hit@qq.com) ; Qi, Wei(wqi@imr.ac.cn) |
2019-06-21 | |
Source Publication | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
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ISSN | 0360-3199 |
Volume | 44Issue:31Pages:16315-16326 |
Abstract | Different density nitrogen vacancy modified g-C3N4 photocatalysts were successfully prepared, and investigated their photocatalytic performance for H-2 evolution and pollutant degradation. In this system, the increase of nitrogen vacancy density could enable the conduction band position of resultant g-C3N4 to negative shift compared to previous g-C3N4. Meanwhile, various positive factors were also introduced in this system, such as larger surface areas, the improvement of light response capacity, effective separation of photogenerated charge, resulting in resultant g-C3N4 photocatalysts exhibiting evident improvement of photocatalytic performance for H-2 evolution and pollutant degradation. Obviously, this work provides physico-chemical insights for the nature of the promotion effect of nitrogen vacancies. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. |
Keyword | g-C3N4 Photocatalyst Nitrogen vacancy H-2 evolution Pollutant degradation |
Funding Organization | talent scientific research fund of LSHU ; basic research projects of Liaoning Provincial Education Department ; NSFC of China |
DOI | 10.1016/j.ijhydene.2019.05.001 |
Indexed By | SCI |
Language | 英语 |
Funding Project | talent scientific research fund of LSHU[2016XJJ-080] ; basic research projects of Liaoning Provincial Education Department[L2017LQN004] ; NSFC of China[21761132010] ; NSFC of China[21573256] ; NSFC of China[91645114] |
WOS Research Area | Chemistry ; Electrochemistry ; Energy & Fuels |
WOS Subject | Chemistry, Physical ; Electrochemistry ; Energy & Fuels |
WOS ID | WOS:000472991100026 |
Publisher | PERGAMON-ELSEVIER SCIENCE LTD |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/134395 |
Collection | 中国科学院金属研究所 |
Corresponding Author | Shi, Lei; Qi, Wei |
Affiliation | 1.Liaoning Shihua Univ, Coll Chem Chem Engn & Environm Engn, Fushun 113001, Peoples R China 2.Shandong Normal Univ, Coll Chem Chem Engn & Mat Sci, Jinan 250014, Shandong, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China |
Recommended Citation GB/T 7714 | Liang, Lei,Shi, Lei,Wang, Fangxiao,et al. Synthesis and photo-catalytic activity of porous g-C3N4: Promotion effect of nitrogen vacancy in H-2 evolution and pollutant degradation reactions[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2019,44(31):16315-16326. |
APA | Liang, Lei,Shi, Lei,Wang, Fangxiao,Yao, Lizhu,Zhang, Ying,&Qi, Wei.(2019).Synthesis and photo-catalytic activity of porous g-C3N4: Promotion effect of nitrogen vacancy in H-2 evolution and pollutant degradation reactions.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,44(31),16315-16326. |
MLA | Liang, Lei,et al."Synthesis and photo-catalytic activity of porous g-C3N4: Promotion effect of nitrogen vacancy in H-2 evolution and pollutant degradation reactions".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44.31(2019):16315-16326. |
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