| Free-standing Monatomic Thick Two-dimensional Gold | |
| Wang, Xuelu1,2; Wang, Chunyang1,3; Chen, Chunjin1,2; Duan, Huichao1,2; Du, Kui1 | |
| Corresponding Author | Du, Kui(kuidu@imr.ac.cn) |
| 2019-07-01 | |
| Source Publication | NANO LETTERS
 |
| ISSN | 1530-6984 |
| Volume | 19Issue:7Pages:4560-4566 |
| Abstract | Monolayer metal membranes have attracted research attention owing to their fascinating physical properties. Unlike layered materials with weak interlayer van der Waals bonding, metallic monolayer membranes are difficult to exfoliate due to strong metallic bonding between layers. Here, we fabricate free-standing monatomic thick Au membranes and nanoribbons framed in bulk crystals using in situ dealloying inside transmission electron microscope. The Au membranes are robust under high energy electron beam. Monatomic-thick nanoribbons with a minimal width of 0.6 nm are observed. First-principles calculations reveal that zigzag-edged nanoribbons are ferromagnetic with magnetic moments ranging 0.38-0.51 mu B per unit-cell for a width less than 0.9 nm. In addition, a linear relationship between the bond length and the coordination number of atoms is directly investigated using atomic resolution images of monolayer and bilayer Au membranes. This work provides a pathway for direct fabrication of metal membranes and nanoribbons and to achieve novel physical properties. |
| Keyword | 2D materials transmission electron microscopy electronic devices dealloying coordination number |
| Funding Organization | National Natural Science Foundation of China ; National Key Research and Development Program of China ; Chinese Academy of Sciences |
| DOI | 10.1021/acs.nanolett.9b01494 |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | National Natural Science Foundation of China[51771203] ; National Key Research and Development Program of China[2017YFA0700701] ; Chinese Academy of Sciences[QYZDJ-SSW-JSC024] |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
| WOS ID | WOS:000475533900044 |
| Publisher | AMER CHEMICAL SOC |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imr.ac.cn/handle/321006/134652 |
| Collection | 中国科学院金属研究所 |
| Corresponding Author | Du, Kui |
| Affiliation | 1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Liaoning, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| Recommended Citation GB/T 7714 | Wang, Xuelu,Wang, Chunyang,Chen, Chunjin,et al. Free-standing Monatomic Thick Two-dimensional Gold[J]. NANO LETTERS,2019,19(7):4560-4566. |
| APA | Wang, Xuelu,Wang, Chunyang,Chen, Chunjin,Duan, Huichao,&Du, Kui.(2019).Free-standing Monatomic Thick Two-dimensional Gold.NANO LETTERS,19(7),4560-4566. |
| MLA | Wang, Xuelu,et al."Free-standing Monatomic Thick Two-dimensional Gold".NANO LETTERS 19.7(2019):4560-4566. |
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