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Thermoelectric performance of a metastable thin-film Heusler alloy
Hinterleitner, B.1,2; Knapp, I.1,2; Poneder, M.1,2; Shi, Yongpeng3,4; Mueller, H.1; Eguchi, G.1; Eisenmenger-Sittner, C.1; Stoeger-Pollach, M.1,5; Kakefuda, Y.6; Kawamoto, N.6; Guo, Q.6,7; Baba, T.6,7; Mori, T.6,7,8; Ullah, Sami3; Chen, Xing-Qiu3,4; Bauer, E.1,2
Corresponding AuthorBauer, E.(bauer@ifp.tuwien.ac.at)
2019-12-05
Source PublicationNATURE
ISSN0028-0836
Volume576Issue:7785Pages:85-+
AbstractThermoelectric materials transform a thermal gradient into electricity. The efficiency of this process relies on three material-dependent parameters:the Seebeck coefficient, the electrical resistivity and the thermal conductivity, summarized in the thermoelectric figure of merit. A large figure of merit is beneficial for potential applications such as thermoelectric generators. Here we report the thermal and electronic properties of thin-film Heusler alloys based on Fe2V0.8W0.2Al prepared by magnetron sputtering. Density functional theory calculations suggest that the thin films are metastable states, and measurements oft he power factor-the ratio of the Seebeck coefficient squared divided by the electrical resistivity-suggest a high intrinsic figure of merit for these thin films. This may arise from a large differential density of states at the Fermi level and a Weyl-like electron dispersion close to the Fermi level, which indicates a high mobility of charge carriers owing to linear crossing in the electronic bands.
Funding OrganizationChristian Doppler Laboratory for Thermoelectricity ; JST, CREST ; National Science Fund for Distinguished Young Scholars ; National Natural Science Foundation of China ; Science Challenging Project ; Shanghai Nuclear Engineering Research & Design Institute
DOI10.1038/s41586-019-1751-9
Indexed BySCI
Language英语
Funding ProjectChristian Doppler Laboratory for Thermoelectricity ; JST, CREST[JPMJCR15Q6] ; JST, CREST[JPMJCR19Q4] ; National Science Fund for Distinguished Young Scholars[51725103] ; National Natural Science Foundation of China[51671193] ; Science Challenging Project[TZ2016004] ; Shanghai Nuclear Engineering Research & Design Institute[2018ZX06002004]
WOS Research AreaScience & Technology - Other Topics
WOS SubjectMultidisciplinary Sciences
WOS IDWOS:000501599200045
PublisherNATURE PUBLISHING GROUP
Citation statistics
Cited Times:85[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/136247
Collection中国科学院金属研究所
Corresponding AuthorBauer, E.
Affiliation1.Tech Univ Wien, Inst Solid State Phys, Vienna, Austria
2.Tech Univ Wien, Christian Doppler Lab Thermoelect, Vienna, Austria
3.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang, Liaoning, Peoples R China
4.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang, Liaoning, Peoples R China
5.Tech Univ Wien, Univ Serv Ctr Transmiss Electron Microscopy, Vienna, Austria
6.NIMS, Int Ctr Mat Nanoarchitecton WPI MANA, Tsukuba, Ibaraki, Japan
7.NIMS, CFSN, Tsukuba, Ibaraki, Japan
8.Univ Tsukuba, Tsukuba, Ibaraki, Japan
Recommended Citation
GB/T 7714
Hinterleitner, B.,Knapp, I.,Poneder, M.,et al. Thermoelectric performance of a metastable thin-film Heusler alloy[J]. NATURE,2019,576(7785):85-+.
APA Hinterleitner, B..,Knapp, I..,Poneder, M..,Shi, Yongpeng.,Mueller, H..,...&Bauer, E..(2019).Thermoelectric performance of a metastable thin-film Heusler alloy.NATURE,576(7785),85-+.
MLA Hinterleitner, B.,et al."Thermoelectric performance of a metastable thin-film Heusler alloy".NATURE 576.7785(2019):85-+.
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