Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting | |
Li, Jing1; Yang, Wenjin1; Wu, Aimin2; Zhang, Xinglai1; Xu, Tingting1; Liu, Baodan1 | |
Corresponding Author | Liu, Baodan(baodanliu@hotmail.com) |
2020-02-19 | |
Source Publication | ACS APPLIED MATERIALS & INTERFACES
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ISSN | 1944-8244 |
Volume | 12Issue:7Pages:8583-8591 |
Abstract | y A (GaN)(1-x)(ZnO)(x) solid solution as a promising visible-light-driven photocatalyst for overall water splitting has attracted extensive attention. In this work, we proposed a template reactive strategy toward the synthesis of band-gap tunable 2D (GaN)(1-x)(ZnO)(x) nanosheets as thin as 14 nm to reduce the carrier transportation path and thus efficiently decrease the recombination of electrons and holes. It is demonstrated that the template strategy enables an ideal morphology and structure transformation from hexagonal 2D ZnGa2O4 nanosheets to 2D (GaN)(1-x)(ZnO)(x) nanosheets in the nitridation process. After the modification of 1 wt % of Rh cocatalyst, the flowerlike (GaN)(0.89)(ZnO)(0.11) nanosheets show an enhanced hydrogen evolution in pure water (pH 4.5). |
Keyword | (GaN)(1-x)(ZnO)(x) solid solution nanosheets photocatalytic water splitting |
Funding Organization | National Natural Science Foundation of China |
DOI | 10.1021/acsami.9b21793 |
Indexed By | SCI |
Language | 英语 |
Funding Project | National Natural Science Foundation of China[51702326] ; National Natural Science Foundation of China[51872296] |
WOS Research Area | Science & Technology - Other Topics ; Materials Science |
WOS Subject | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS ID | WOS:000515214300079 |
Publisher | AMER CHEMICAL SOC |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/137328 |
Collection | 中国科学院金属研究所 |
Corresponding Author | Liu, Baodan |
Affiliation | 1.Chinese Acad Sci, IMR, Shenyang Natl Lab Mat Sci SYNL, Shenyang 110016, Peoples R China 2.Dalian Univ Technol, Key Lab Mat Modificat Laser Ion & Elect Beams, Minist Educ, Dalian 116024, Peoples R China |
Recommended Citation GB/T 7714 | Li, Jing,Yang, Wenjin,Wu, Aimin,et al. Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting[J]. ACS APPLIED MATERIALS & INTERFACES,2020,12(7):8583-8591. |
APA | Li, Jing,Yang, Wenjin,Wu, Aimin,Zhang, Xinglai,Xu, Tingting,&Liu, Baodan.(2020).Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting.ACS APPLIED MATERIALS & INTERFACES,12(7),8583-8591. |
MLA | Li, Jing,et al."Band-Gap Tunable 2D Hexagonal (GaN)(1-x)(ZnO)(x) Solid-Solution Nanosheets for Photocatalytic Water Splitting".ACS APPLIED MATERIALS & INTERFACES 12.7(2020):8583-8591. |
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