Oxidation and cracking/spallation resistance of ZrB2-SiC-TaSi2-Si coating on siliconized graphite at 1500 degrees C in air

doi:10.1016/j.ceramint.2019.11.095

IMR OpenIR

	Oxidation and cracking/spallation resistance of ZrB2-SiC-TaSi2-Si coating on siliconized graphite at 1500 degrees C in air
	Ren, Yan 1,2; Qian, Yuhai 1; Xu, Jingjun 1; Jiang, Yan 3,4; Zuo, Jun 1; Li, Meishuan 1
通讯作者	Qian, Yuhai(yhqian@imr.ac.cn)
	2020-04-01
发表期刊	CERAMICS INTERNATIONAL
ISSN	0272-8842
卷号	46 期号:5 页码:6254-6261
摘要	A ZrB2-SiC-TaSi2-Si coating on siliconized graphite substrate was prepared by a combination process of slurry brushing and vapor silicon infiltration. The high-temperature oxidation behavior and cracking/spallation resistance of the as-prepared coating were investigated in detail. It was revealed that the oxidation kinetics at 1500 degrees C in static air followed a parabolic law with a relatively low oxidation rate constant down to 0.27 mg/(cm(2).h(0.5)). The crack area ratio of the as-prepared coating was determined as 3.8 x 10(-3) after severe thermal cycling from 1500 degrees C to room temperature for 20 times. Apart from the formation of ZrO2 as skeleton phase with SiO2 as infilling species, the good oxidation and cracking/spallation resistance of the coating also could be attributed to its unique duplex-layered structure, i.e., a dense ZrB2-SiC-TaSi2-Si major layer filled with Si and an outermost Si cladding top layer. Meanwhile, the strong adhesion strength of the SiC transition layer with the graphite substrate and the outer ZrB2-SiC-TaSi2-Si layer was a vital factor as well.
关键词	Coating Oxidation resistance ZrB2-SiC-TaSi2 Vapor silicon infiltration
资助者	National Natural Science Foundation of China
DOI	10.1016/j.ceramint.2019.11.095
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51571203] ; National Natural Science Foundation of China[51571205]
WOS研究方向	Materials Science
WOS类目	Materials Science, Ceramics
WOS记录号	WOS:000515196800091
出版者	ELSEVIER SCI LTD
引用统计	被引频次：26[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/137547
专题	中国科学院金属研究所
通讯作者	Qian, Yuhai
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 3.Northeastern Univ, Key Lab Anisotropy & Texture Mat, Minist Educ, Shenyang 110819, Peoples R China 4.Northeastern Univ, Sch Mat Sci & Engn, Inst Ceram & Powder Met, Shenyang 110819, Peoples R China
推荐引用方式 GB/T 7714	Ren, Yan,Qian, Yuhai,Xu, Jingjun,et al. Oxidation and cracking/spallation resistance of ZrB2-SiC-TaSi2-Si coating on siliconized graphite at 1500 degrees C in air[J]. CERAMICS INTERNATIONAL,2020,46(5):6254-6261.
APA	Ren, Yan,Qian, Yuhai,Xu, Jingjun,Jiang, Yan,Zuo, Jun,&Li, Meishuan.(2020).Oxidation and cracking/spallation resistance of ZrB2-SiC-TaSi2-Si coating on siliconized graphite at 1500 degrees C in air.CERAMICS INTERNATIONAL,46(5),6254-6261.
MLA	Ren, Yan,et al."Oxidation and cracking/spallation resistance of ZrB2-SiC-TaSi2-Si coating on siliconized graphite at 1500 degrees C in air".CERAMICS INTERNATIONAL 46.5(2020):6254-6261.