Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol

doi:10.1016/j.cplett.2020.137306

IMR OpenIR

	Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol
	Zhao, Zhiliang 1; Zhang, Jing 1; Wang, Yongzhao 2; Guo, Wenyao 1; Lv, Lin 1; Li, Baiyu 3; Zheng, Kang 1; Bo, Tingting 1; Peng, Dengchao 1; Zhou, Zhiyuan 1; Zhang, Bingsen 2; Shao, Lidong 1
通讯作者	Guo, Wenyao(guowenyao@shiep.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
	2020-05-01
发表期刊	CHEMICAL PHYSICS LETTERS
ISSN	0009-2614
卷号	746 页码:6
摘要	In this work, Pd/reduced graphene oxide (Pd/RGO) aerogels, with large surface areas and wrinkles, are obtained through the lyophilisation, vacuum and reduction treatments. Pd/RGO aerogels exhibit higher catalytic performances and thermal stability in comparison to the reference catalyst Pd/activated carbon (Pd/AC) in the oxidation of benzyl alcohol. The surface analyses indicate that Pd/RGO aerogels possess a higher proportion of Pd2+ than the Pd/AC catalyst. Meanwhile, the oxygen-containing functional groups can modulate the interaction between palladium and the support to form active phases for the reaction. Moreover, Pd nanoparticles (PdNPs) remain well dispersed in nanoscale on the reacted Pd/RGO aerogels.
关键词	Pd nanoparticles Solvent-free oxidation Benzyl alcohol Graphene oxide Aerogel
资助者	National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program
DOI	10.1016/j.cplett.2020.137306
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[21773269] ; Liao Ning Revitalization Talents Program[XLYC1807175]
WOS研究方向	Chemistry ; Physics
WOS类目	Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS记录号	WOS:000522555600027
出版者	ELSEVIER
引用统计	被引频次：16[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/137851
专题	中国科学院金属研究所
通讯作者	Guo, Wenyao; Zhang, Bingsen; Shao, Lidong
作者单位	1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China 2.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China 3.Nantong Vocat Univ, 89 Qingnian Rd, Nantong 226006, Peoples R China
推荐引用方式 GB/T 7714	Zhao, Zhiliang,Zhang, Jing,Wang, Yongzhao,et al. Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol[J]. CHEMICAL PHYSICS LETTERS,2020,746:6.
APA	Zhao, Zhiliang.,Zhang, Jing.,Wang, Yongzhao.,Guo, Wenyao.,Lv, Lin.,...&Shao, Lidong.(2020).Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol.CHEMICAL PHYSICS LETTERS,746,6.
MLA	Zhao, Zhiliang,et al."Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol".CHEMICAL PHYSICS LETTERS 746(2020):6.