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Vertically Oriented Topological Insulator Bi2Se3 Nanoplates on Silicon for Broadband Photodetection
Li, Mingze1,2; Wang, Zhenhua1,2; Gao, Xuan P. A.3; Zhang, Zhidong1,2
通讯作者Wang, Zhenhua(zhwang@imr.ac.cn) ; Gao, Xuan P. A.(xuan.gao@case.edu)
2020-05-07
发表期刊JOURNAL OF PHYSICAL CHEMISTRY C
ISSN1932-7447
卷号124期号:18页码:10135-10142
摘要As an exotic state of quantum matter, topological insulators like Bi2Se3 have potential applications in low power electronic and optoelectronic devices. Bi2Se3 nanoflakes or films with (001) orientation, laying horizontally on substrates, have been studied extensively in the past few years. Here we report the growth and photodetection response of Bi2Se3 nanoplates oriented vertically on the p-type Si substrate. This unconventional structure and geometry provide a higher effective absorption length for light absorption and potentially more efficient photocarrier transport via the topologically protected surface states or the basal plane of Bi2Se3 nanoplates. By compensating Bi2Se3 native defects with Cu doping, we achieve an increase of 42 times in the photocurrent when the Cu concentration is 3.87 at. %. Our work paves a way for exploring the excellent optoelectronic properties of topological insulator films with an unconventional orientation.
资助者National Natural Science Foundation of China (NSFC) ; National Key R&D Program of China ; Foundation of National Laboratory for Materials Science ; Liaoning Revitalization Talents Program ; United Foundation of Liaoning Province and National Laboratory for Materials Science
DOI10.1021/acs.jpcc.0c01978
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China (NSFC)[51971220] ; National Key R&D Program of China[2017YFA0206302] ; Foundation of National Laboratory for Materials Science[L2019R31] ; Liaoning Revitalization Talents Program[XLYC1807122] ; United Foundation of Liaoning Province and National Laboratory for Materials Science[2019JH3]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000535175400051
出版者AMER CHEMICAL SOC
引用统计
被引频次:17[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/138985
专题中国科学院金属研究所
通讯作者Wang, Zhenhua; Gao, Xuan P. A.
作者单位1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
2.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Peoples R China
3.Case Western Reserve Univ, Dept Phys, Cleveland, OH 44106 USA
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Li, Mingze,Wang, Zhenhua,Gao, Xuan P. A.,et al. Vertically Oriented Topological Insulator Bi2Se3 Nanoplates on Silicon for Broadband Photodetection[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2020,124(18):10135-10142.
APA Li, Mingze,Wang, Zhenhua,Gao, Xuan P. A.,&Zhang, Zhidong.(2020).Vertically Oriented Topological Insulator Bi2Se3 Nanoplates on Silicon for Broadband Photodetection.JOURNAL OF PHYSICAL CHEMISTRY C,124(18),10135-10142.
MLA Li, Mingze,et al."Vertically Oriented Topological Insulator Bi2Se3 Nanoplates on Silicon for Broadband Photodetection".JOURNAL OF PHYSICAL CHEMISTRY C 124.18(2020):10135-10142.
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