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Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3
Zheng, Kang1; Zhou, Zhiyuan1; Wang, Yongzhao2; Xin, Zhiling1; Zhao, Zhiliang1; Zhang, Jing1; Bo, Tingting1; Lin, Tsungwu3; Zhang, Bingsen2; Shao, Lidong1
Corresponding AuthorXin, Zhiling(xinzhiling@126.com) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
2020-05-21
Source PublicationCATALYSIS SCIENCE & TECHNOLOGY
ISSN2044-4753
Volume10Issue:10Pages:3450-3457
AbstractWe report a facile method for dispersing Mn species onto two-dimensional Co3O4 nanosheets at the nanoscale for the selective catalytic reduction (SCR) of NOx with NH3. In comparison with the reference catalysts with higher Mn loadings, the Mn/Co3O4 (0.8 wt%) catalyst exhibits improved catalytic activity and a high H2O-resistance ability. Due to the strong interaction between cobalt and manganese oxides and the increased surface area of the Co3O4 nanosheets, the catalyst with an ultralow amount of Mn at the nanoscale possesses stronger reducibility, abundant Co3+ and surface oxygen species, which in turn enhance the NH3-SCR activity.
Funding OrganizationScience and Technology Commission of Shanghai Municipality ; National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program ; Research Fund of SYNL
DOI10.1039/d0cy00599a
Indexed BySCI
Language英语
Funding ProjectScience and Technology Commission of Shanghai Municipality[19DZ2271100] ; National Natural Science Foundation of China[21761132025] ; Liao Ning Revitalization Talents Program[XLYC1807175] ; Research Fund of SYNL[L2019F38]
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000538156300026
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/139101
Collection中国科学院金属研究所
Corresponding AuthorXin, Zhiling; Zhang, Bingsen; Shao, Lidong
Affiliation1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China
3.Tunghai Univ, Dept Chem, 181,Sec 3,Port Rd, Taichung 40704, Taiwan
Recommended Citation
GB/T 7714
Zheng, Kang,Zhou, Zhiyuan,Wang, Yongzhao,et al. Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3[J]. CATALYSIS SCIENCE & TECHNOLOGY,2020,10(10):3450-3457.
APA Zheng, Kang.,Zhou, Zhiyuan.,Wang, Yongzhao.,Xin, Zhiling.,Zhao, Zhiliang.,...&Shao, Lidong.(2020).Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3.CATALYSIS SCIENCE & TECHNOLOGY,10(10),3450-3457.
MLA Zheng, Kang,et al."Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3".CATALYSIS SCIENCE & TECHNOLOGY 10.10(2020):3450-3457.
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