Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3

doi:10.1039/d0cy00599a

IMR OpenIR

	Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3
	Zheng, Kang 1; Zhou, Zhiyuan 1; Wang, Yongzhao 2; Xin, Zhiling 1; Zhao, Zhiliang 1; Zhang, Jing 1; Bo, Tingting 1; Lin, Tsungwu 3; Zhang, Bingsen 2; Shao, Lidong 1
Corresponding Author	Xin, Zhiling(xinzhiling@126.com) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
	2020-05-21
Source Publication	CATALYSIS SCIENCE & TECHNOLOGY
ISSN	2044-4753
Volume	10 Issue:10 Pages:3450-3457
Abstract	We report a facile method for dispersing Mn species onto two-dimensional Co3O4 nanosheets at the nanoscale for the selective catalytic reduction (SCR) of NOx with NH3. In comparison with the reference catalysts with higher Mn loadings, the Mn/Co3O4 (0.8 wt%) catalyst exhibits improved catalytic activity and a high H2O-resistance ability. Due to the strong interaction between cobalt and manganese oxides and the increased surface area of the Co3O4 nanosheets, the catalyst with an ultralow amount of Mn at the nanoscale possesses stronger reducibility, abundant Co3+ and surface oxygen species, which in turn enhance the NH3-SCR activity.
Funding Organization	Science and Technology Commission of Shanghai Municipality ; National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program ; Research Fund of SYNL
DOI	10.1039/d0cy00599a
Indexed By	SCI
Language	英语
Funding Project	Science and Technology Commission of Shanghai Municipality[19DZ2271100] ; National Natural Science Foundation of China[21761132025] ; Liao Ning Revitalization Talents Program[XLYC1807175] ; Research Fund of SYNL[L2019F38]
WOS Research Area	Chemistry
WOS Subject	Chemistry, Physical
WOS ID	WOS:000538156300026
Publisher	ROYAL SOC CHEMISTRY
Citation statistics	Cited Times:10[WOS] [WOS Record] [Related Records in WOS]
Document Type	期刊论文
Identifier	http://ir.imr.ac.cn/handle/321006/139101
Collection	中国科学院金属研究所
Corresponding Author	Xin, Zhiling; Zhang, Bingsen; Shao, Lidong
Affiliation	1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China 3.Tunghai Univ, Dept Chem, 181,Sec 3,Port Rd, Taichung 40704, Taiwan
Recommended Citation GB/T 7714	Zheng, Kang,Zhou, Zhiyuan,Wang, Yongzhao,et al. Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3[J]. CATALYSIS SCIENCE & TECHNOLOGY,2020,10(10):3450-3457.
APA	Zheng, Kang.,Zhou, Zhiyuan.,Wang, Yongzhao.,Xin, Zhiling.,Zhao, Zhiliang.,...&Shao, Lidong.(2020).Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3.CATALYSIS SCIENCE & TECHNOLOGY,10(10),3450-3457.
MLA	Zheng, Kang,et al."Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3".CATALYSIS SCIENCE & TECHNOLOGY 10.10(2020):3450-3457.

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