Recent progress on the recycling technology of Li-ion batteries
Wang, Yuqing1; An, Ning1; Wen, Lei2; Wang, Lei1; Jiang, Xiaotong3; Hou, Feng1; Yin, Yuxin4; Liang, Ji1,5
Corresponding AuthorHou, Feng( ; Liang, Ji(
AbstractLithium-ion batteries (LIBs) have been widely applied in portable electronic devices and electric vehicles. With the booming of the respective markets, a huge quantity of spent LIBs that typically use either LiFePO4 or LiNixCoyMnzO2 cathode materials will be produced in the very near future, imposing significant pressure for the development of suitable disposal/recycling technologies, in terms of both environmental protection and resource reclaiming. In this review, we firstly do a comprehensive summary of the-state-of-art technologies to recycle LiNixCoyMnzO2 and LiFePO4-based LIBs, in the aspects of pretreatment, hydrometallurgical recycling, and direct regeneration of the cathode materials. This closed-loop strategy for cycling cathode materials has been regarded as an ideal approach considering its economic benefit and environmental friendliness. Afterward, as for the exhausted anode materials, we focus on the utilization of exhausted anode materials to obtain other functional materials, such as graphene. Finally, the existing challenges in recycling the LiFePO4 and LiNixCoyMnzO2 cathodes and graphite anodes for industrial-scale application are discussed in detail; and the possible strategies for these issues are proposed. We expect this review can provide a roadmap towards better technologies for recycling LIBs, shed light on the future development of novel battery recycling technologies to promote the environmental benignity and economic viability of the battery industry and pave way for the large-scale application of LIBs in industrial fields in the near future. (C) 2020 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
KeywordLi ion battery Recycling Cathode Anode
Funding OrganizationNational Natural Science Foundation of China ; Australian Research Council (ARC) through Discovery Early Career Researcher Award (DECRA) program
Indexed BySCI
Funding ProjectNational Natural Science Foundation of China[51072130] ; National Natural Science Foundation of China[51502045] ; National Natural Science Foundation of China[21905202] ; Australian Research Council (ARC) through Discovery Early Career Researcher Award (DECRA) program[DE170100871]
WOS Research AreaChemistry ; Energy & Fuels ; Engineering
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS IDWOS:000605241500006
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Cited Times:51[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Corresponding AuthorHou, Feng; Liang, Ji
Affiliation1.Tianjin Univ, Sch Mat Sci & Engn, Key Lab Adv Ceram & Machining Technol, Minist Educ, Tianjin 300072, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
3.China Automot Technol & Res Ctr Co Ltd, Tianjin 300300, Peoples R China
4.Tianjin Lishen Battery Joint Stock Ltd Co, Tianjin 300384, Peoples R China
5.Univ Wollongong, Inst Superconducting & Elect Mat, Australian Inst Innovat Mat, Innovat Campus, North Wollongong, NSW 2500, Australia
Recommended Citation
GB/T 7714
Wang, Yuqing,An, Ning,Wen, Lei,et al. Recent progress on the recycling technology of Li-ion batteries[J]. JOURNAL OF ENERGY CHEMISTRY,2021,55:391-419.
APA Wang, Yuqing.,An, Ning.,Wen, Lei.,Wang, Lei.,Jiang, Xiaotong.,...&Liang, Ji.(2021).Recent progress on the recycling technology of Li-ion batteries.JOURNAL OF ENERGY CHEMISTRY,55,391-419.
MLA Wang, Yuqing,et al."Recent progress on the recycling technology of Li-ion batteries".JOURNAL OF ENERGY CHEMISTRY 55(2021):391-419.
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