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Nanoscale Pd Supported on Layered Co(OH)(2) as Efficient Catalysts for Solvent-Free Oxidation of Benzyl Alcohol
Lv, Lin1; Wang, Yongzhao2; Peng, Dengchao1; Zhou, Zhiyuan1; Shang, Jing1; Guo, Wenyao1; Zhang, Bingsen2; Xin, Zhiling1
Corresponding AuthorGuo, Wenyao(guowenyao@shiep.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Xin, Zhiling(xinzhiling@126.com)
2021-08-06
Source PublicationCHEMISTRYSELECT
ISSN2365-6549
Volume6Issue:29Pages:7384-7390
AbstractIn this work, two-dimensional (2D) Co(OH)(2) nanosheets, with large surface areas and wrinkles are obtained, and used to support Pd nanoparticles (NPs) by simple impregnation method as an efficient catalyst for the oxidation of benzyl alcohol under solvent-free conditions. The resulting 1 wt.% Pd/Co(OH)(2) catalyst exhibits a high turnover frequency value of 57999 h(-1). The catalysts were characterized by SEM, TEM, AFM, XRD, BET, XPS and CO-pulse chemisorption. The results of characterizations reveal that the Pd NPs are highly dispersed on the Co(OH)(2) nanosheets. The abundant hydroxyl groups on the surface of Co(OH)(2) nanosheets promote the reduction of Pd species, resulting in a higher proportion of Pd-0 than that of Pd/AC catalyst, which further facilitates the catalytic performances.
KeywordBenzyl alcohol Layered Co(OH)(2) Oxidation Pd nanoparticles Supported catalysts
Funding OrganizationNational Natural Science Foundation of China ; Liao Ning Revitalization Talents Program
DOI10.1002/slct.202101673
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[21773269] ; Liao Ning Revitalization Talents Program[XLYC1807175]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000680162200016
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/159313
Collection中国科学院金属研究所
Corresponding AuthorGuo, Wenyao; Zhang, Bingsen; Xin, Zhiling
Affiliation1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, Shanghai 200090, Peoples R China
2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
Recommended Citation
GB/T 7714
Lv, Lin,Wang, Yongzhao,Peng, Dengchao,et al. Nanoscale Pd Supported on Layered Co(OH)(2) as Efficient Catalysts for Solvent-Free Oxidation of Benzyl Alcohol[J]. CHEMISTRYSELECT,2021,6(29):7384-7390.
APA Lv, Lin.,Wang, Yongzhao.,Peng, Dengchao.,Zhou, Zhiyuan.,Shang, Jing.,...&Xin, Zhiling.(2021).Nanoscale Pd Supported on Layered Co(OH)(2) as Efficient Catalysts for Solvent-Free Oxidation of Benzyl Alcohol.CHEMISTRYSELECT,6(29),7384-7390.
MLA Lv, Lin,et al."Nanoscale Pd Supported on Layered Co(OH)(2) as Efficient Catalysts for Solvent-Free Oxidation of Benzyl Alcohol".CHEMISTRYSELECT 6.29(2021):7384-7390.
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