| Electrocatalytic-driven compensation for sodium ion pouch cell with high energy density and long lifespan | |
| Zhang, Qi1,3,4; Gao, Xuan-Wen1; Shi, Ying2; Luo, Wen-Bin1; Li, Yang3; Gu, Qin-Fen1; Fan, Hai-Ning3; Li, Feng2; Liu, Hua-Kun3 | |
| Corresponding Author | Luo, Wen-Bin(luowenbin@smm.neu.edu.cn) ; Gu, Qin-Fen(qinfeng@ansto.gov.au) ; Li, Feng(fli@imr.ac.cn) |
| 2021-08-01 | |
| Source Publication | ENERGY STORAGE MATERIALS
 |
| ISSN | 2405-8297 |
| Volume | 39Pages:54-59 |
| Abstract | The content of cyclable sodium ions in the sodium ion pouch cell can determine the energy density and cycling lifespan directly and efficiently by alleviating the sodium ion loss in the initial formation process and following cycling period. The method of electrocatalytic-driven compensation sodium ions was explored, and the cell fabrication process was proposed as well. High sodium content (88%) sodium oxide (Na2O) can provide sufficient cyclable sodium ions electrocatalytic-driven by high active Ruthenium@graphene (Ru@G) electrocatalyst to compensate the sodium loss during the initial solid electrolyte layer formation and following consumption. This electrocatalytic-driven compensation can provide numerous cyclable sodium, but also be no adverse effects on the stability of electrode materials, electrolyte, and the whole battery. Meanwhile, the industrial feasibility of this cell fabrication process can accelerate the practical application. Based on this technology, the initial coulombic efficiency of pouch cell can reach up to 90%, while the 295 Wh Kg(-1) materials energy density is much superior and promising for future energy storage system application. |
| Keyword | Sodium compensation Sodium ion battery Electrocatalyst Sodium oxide Cathode materials |
| Funding Organization | Fundamental Research Funds for the Central Universities ; China Scholarship Council ; PD beamline at the Australian Synchrotron, ANSTO |
| DOI | 10.1016/j.ensm.2021.04.011 |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | Fundamental Research Funds for the Central Universities[N2025018] ; Fundamental Research Funds for the Central Universities[N2025009] ; China Scholarship Council ; PD beamline at the Australian Synchrotron, ANSTO |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science |
| WOS Subject | Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
| WOS ID | WOS:000658385000005 |
| Publisher | ELSEVIER |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imr.ac.cn/handle/321006/160429 |
| Collection | 中国科学院金属研究所 |
| Corresponding Author | Luo, Wen-Bin; Gu, Qin-Fen; Li, Feng |
| Affiliation | 1.Northeastern Univ, Sch Met, Inst Energy Electrochem & Urban Mines Met, 11 Lane 3,Wenhua Rd, Shenyang, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang, Peoples R China 3.Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia 4.Taiyuan Univ Technol, Coll Mech & Vehicle Engn, Taiyuan 030024, Peoples R China |
| Recommended Citation GB/T 7714 | Zhang, Qi,Gao, Xuan-Wen,Shi, Ying,et al. Electrocatalytic-driven compensation for sodium ion pouch cell with high energy density and long lifespan[J]. ENERGY STORAGE MATERIALS,2021,39:54-59. |
| APA | Zhang, Qi.,Gao, Xuan-Wen.,Shi, Ying.,Luo, Wen-Bin.,Li, Yang.,...&Liu, Hua-Kun.(2021).Electrocatalytic-driven compensation for sodium ion pouch cell with high energy density and long lifespan.ENERGY STORAGE MATERIALS,39,54-59. |
| MLA | Zhang, Qi,et al."Electrocatalytic-driven compensation for sodium ion pouch cell with high energy density and long lifespan".ENERGY STORAGE MATERIALS 39(2021):54-59. |
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