Hierarchical thermal transport mechanisms in Yb2Si2O7 multifunctional thermal and environmental barrier coating (TEBC) material | |
Luo, Yixiu1; Yang, Xiaolong2; Wang, Jingyang1 | |
通讯作者 | Wang, Jingyang(jywang@imr.ac.cn) |
2021-03-15 | |
发表期刊 | SCRIPTA MATERIALIA
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ISSN | 1359-6462 |
卷号 | 194页码:5 |
摘要 | Understanding the mechanism of thermal conduction and its modulation strategy is a threshold task in the search of advanced multifunctional thermal and environmental barrier coating materials (TEBCs). We herein disclose the hierarchical features in the thermal transport of a typical TEBC material, Yb2Si2O7, using the state-of-the-art dual-phonon theory. Large amounts of vibrational modes transport heat in a diffusive feature, different from the propagative feature for normal phonons, and make significant contribution to the lattice thermal conductivity (kappa(L)) at high temperatures (T). This mechanism drives a weak kappa(L)similar to T dependence at high temperatures, deviating from the kappa(L)similar to T-1 trend predicted by the phonon Boltzmann transport equation (BTE) theory. The present study indicates that modulating the kappa L-L of complex-structure low-kappa(L) TEBC materials requires wisdoms beyond the BTE theory and considering the joint effects from different thermal transport channels. (c) 2020 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. |
关键词 | Ceramic Thermal conductivity Modeling Phonon engineering |
资助者 | National Science and Technology Major Project ; Natural Science Foundation of China ; CAS International Cooperation Key Program ; Shenyang National Laboratory for Materials Science |
DOI | 10.1016/j.scriptamat.2020.113704 |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Science and Technology Major Project[2017-VI-0020-0093] ; Natural Science Foundation of China[51772302] ; CAS International Cooperation Key Program[174321KYSB20180008] ; Shenyang National Laboratory for Materials Science[L2019F22] |
WOS研究方向 | Science & Technology - Other Topics ; Materials Science ; Metallurgy & Metallurgical Engineering |
WOS类目 | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering |
WOS记录号 | WOS:000613278700016 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.imr.ac.cn/handle/321006/160511 |
专题 | 中国科学院金属研究所 |
通讯作者 | Wang, Jingyang |
作者单位 | 1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Shenzhen Univ, Inst Adv Study, Shenzhen 518060, Peoples R China |
推荐引用方式 GB/T 7714 | Luo, Yixiu,Yang, Xiaolong,Wang, Jingyang. Hierarchical thermal transport mechanisms in Yb2Si2O7 multifunctional thermal and environmental barrier coating (TEBC) material[J]. SCRIPTA MATERIALIA,2021,194:5. |
APA | Luo, Yixiu,Yang, Xiaolong,&Wang, Jingyang.(2021).Hierarchical thermal transport mechanisms in Yb2Si2O7 multifunctional thermal and environmental barrier coating (TEBC) material.SCRIPTA MATERIALIA,194,5. |
MLA | Luo, Yixiu,et al."Hierarchical thermal transport mechanisms in Yb2Si2O7 multifunctional thermal and environmental barrier coating (TEBC) material".SCRIPTA MATERIALIA 194(2021):5. |
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