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Dissolution-precipitation growth of uniform and clean two dimensional transition metal dichalcogenides
Cai, Zhengyang1,2; Lai, Yongjue1,2; Zhao, Shilong1,2; Zhang, Rongjie1,2; Tan, Junyang1,2; Feng, Simin1,2; Zou, Jingyun1,2; Tang, Lei1,2; Lin, Junhao4; Liu, Bilu1,2; Cheng, Hui-Ming1,2,3
Corresponding AuthorLiu, Bilu(bilu.liu@sz.tsinghua.edu.cn) ; Cheng, Hui-Ming(cheng@imr.ac.cn)
2021-03-01
Source PublicationNATIONAL SCIENCE REVIEW
ISSN2095-5138
Volume8Issue:3Pages:9
AbstractTwo dimensional transition metal dichalcogenides (TMDCs) have attracted much interest and shown promise in many applications. However, it is challenging to obtain uniform TMDCs with clean surfaces, because of the difficulties in controlling the way the reactants are supplied to the reaction in the current chemical vapor deposition growth process. Here, we report a new growth approach called `dissolution-precipitation' (DP) growth, where the metal sources are sealed inside glass substrates to control their feeding to the reaction. Noteworthy, the diffusion of metal source inside glass to its surface provides a uniform metal source on the glass surface, and restricts the TMDC growth to only a surface reaction while eliminating unwanted gas-phase reaction. This feature gives rise to highly uniform monolayer TMDCs with a clean surface on centimeter-scale substrates. The DP growth works well for a large variety of TMDCs and their alloys, providing a solid foundation for the controlled growth of clean TMDCs by the fine control of the metal source.
Keyworddissolution-precipitation growth two dimensional materials transition metal dichalcogenides uniform clean
Funding OrganizationNational Natural Science Foundation of China ; Youth 1000-Talent Program of China ; National Key RD Program ; Guangdong Innovative and Entrepreneurial Research Team Program ; Guandong International Science Collaboration Project ; Bureau of Industry and Information Technology of Shenzhen ; Development and Reform Commission of Shenzhen Municipality ; Presidential fund
DOI10.1093/nsr/nwaa115
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51722206] ; National Natural Science Foundation of China[51991340] ; National Natural Science Foundation of China[51991343] ; National Natural Science Foundation of China[11974156] ; National Natural Science Foundation of China[51920105002] ; Youth 1000-Talent Program of China ; National Key RD Program[2018YFA0307200] ; Guangdong Innovative and Entrepreneurial Research Team Program[2017ZT07C341] ; Guandong International Science Collaboration Project[2019A050510001] ; Bureau of Industry and Information Technology of Shenzhen[201901171523] ; Development and Reform Commission of Shenzhen Municipality ; Presidential fund
WOS Research AreaScience & Technology - Other Topics
WOS SubjectMultidisciplinary Sciences
WOS IDWOS:000649002700006
PublisherOXFORD UNIV PRESS
Citation statistics
Cited Times:13[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/160820
Collection中国科学院金属研究所
Corresponding AuthorLiu, Bilu; Cheng, Hui-Ming
Affiliation1.Tsinghua Univ, Shenzhen Geim Graphene Ctr, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China
2.Tsinghua Univ, Tsinghua Shenzher Int Grad Sch, Shenzhen 518055, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
4.Southern Univ Sci & Technol, Dept Phys, Shenzhen 518055, Peoples R China
Recommended Citation
GB/T 7714
Cai, Zhengyang,Lai, Yongjue,Zhao, Shilong,et al. Dissolution-precipitation growth of uniform and clean two dimensional transition metal dichalcogenides[J]. NATIONAL SCIENCE REVIEW,2021,8(3):9.
APA Cai, Zhengyang.,Lai, Yongjue.,Zhao, Shilong.,Zhang, Rongjie.,Tan, Junyang.,...&Cheng, Hui-Ming.(2021).Dissolution-precipitation growth of uniform and clean two dimensional transition metal dichalcogenides.NATIONAL SCIENCE REVIEW,8(3),9.
MLA Cai, Zhengyang,et al."Dissolution-precipitation growth of uniform and clean two dimensional transition metal dichalcogenides".NATIONAL SCIENCE REVIEW 8.3(2021):9.
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