Bottom-Up Approach Derived Iron and Nitrogen Cofunctionalized Carbon as Efficient Renewable Catalyst for Selective Reduction of Nitroarenes | |
Wu, Shuchang3; Wen, Guodong1; Su, Yang2; Pan, Xiaoli2; Yan, Hua3; Diao, Jiangyong1; Liu, Hongyang1 | |
Corresponding Author | Wu, Shuchang(scwu10b@alum.imr.ac.cn) ; Diao, Jiangyong(jydiao@imr.ac.cn) ; Liu, Hongyang(liuhy@imr.ac.cn) |
2021-03-11 | |
Source Publication | JOURNAL OF PHYSICAL CHEMISTRY C
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ISSN | 1932-7447 |
Volume | 125Issue:9Pages:5127-5135 |
Abstract | The non-noble metal and nitrogen cofunctionalized carbon (M-N-C) attract enormous attentions in heterogeneous catalysis. However, the fabrication of the M-N-C systems commonly rely on fossil resource based carbon, while the exploitation of biomass derived materials often suffer from issues such as tedious procedures, complex composition of the biomass and excessive dosage of the dopant precursor. In this study, a direct and large-scale, bottom-up method was developed for the fabrication of the sustainable iron and nitrogen cofunctionalized carbon (FeNC) in a green and sustainable way. The obtained FeNC possessed well-defined structure as well as uniformly distributed iron species. The catalytic results suggested that FeNC could serve as efficient catalyst for the selective reduction of nitroarenes. The FeNx species played an important role, while the N-doped carbon matrix may also involve in the reaction. |
Funding Organization | National Key R&D Program of China ; National Natural Science Foundation of China ; Liaoning Revitalization Talents Program ; Sinopec China ; Guangxi Key Laboratory of Information Materials (Guilin University of Electronic Technology) ; Zhejiang Provincial Natural Science Foundation of China ; Taizhou Science and Technology Planning Project |
DOI | 10.1021/acs.jpcc.1c00620 |
Indexed By | SCI |
Language | 英语 |
Funding Project | National Key R&D Program of China[2016YFA0204100] ; National Natural Science Foundation of China[91845201] ; National Natural Science Foundation of China[21961160722] ; National Natural Science Foundation of China[21703261] ; Liaoning Revitalization Talents Program[XLYC1907055] ; Sinopec China ; Guangxi Key Laboratory of Information Materials (Guilin University of Electronic Technology)[191005-K] ; Zhejiang Provincial Natural Science Foundation of China[LQ20B060001] ; Taizhou Science and Technology Planning Project[1902gy20] |
WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science |
WOS Subject | Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS ID | WOS:000629169900022 |
Publisher | AMER CHEMICAL SOC |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.imr.ac.cn/handle/321006/161547 |
Collection | 中国科学院金属研究所 |
Corresponding Author | Wu, Shuchang; Diao, Jiangyong; Liu, Hongyang |
Affiliation | 1.Chinese Acad Sci, Inst Met Res, Shenyang 110016, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 3.Taizhou Univ, Sch Pharmaceut & Mat Engn, Taizhou 318000, Zhejiang, Peoples R China |
Recommended Citation GB/T 7714 | Wu, Shuchang,Wen, Guodong,Su, Yang,et al. Bottom-Up Approach Derived Iron and Nitrogen Cofunctionalized Carbon as Efficient Renewable Catalyst for Selective Reduction of Nitroarenes[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2021,125(9):5127-5135. |
APA | Wu, Shuchang.,Wen, Guodong.,Su, Yang.,Pan, Xiaoli.,Yan, Hua.,...&Liu, Hongyang.(2021).Bottom-Up Approach Derived Iron and Nitrogen Cofunctionalized Carbon as Efficient Renewable Catalyst for Selective Reduction of Nitroarenes.JOURNAL OF PHYSICAL CHEMISTRY C,125(9),5127-5135. |
MLA | Wu, Shuchang,et al."Bottom-Up Approach Derived Iron and Nitrogen Cofunctionalized Carbon as Efficient Renewable Catalyst for Selective Reduction of Nitroarenes".JOURNAL OF PHYSICAL CHEMISTRY C 125.9(2021):5127-5135. |
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