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Fully Exposed Cluster Catalyst (FECC): Toward Rich Surface Sites and Full Atom Utilization Efficiency
Peng, Mi1,2,3; Dong, Chunyang1,2,3; Gao, Rui4; Xiao, Dequan5; Liu, Hongyang6; Ma, Ding1,2,3
Corresponding AuthorLiu, Hongyang(liuhy@imr.ac.cn) ; Ma, Ding(dma@pku.edu.cn)
2021-02-24
Source PublicationACS CENTRAL SCIENCE
ISSN2374-7943
Volume7Issue:2Pages:262-273
AbstractIncreasing attention has been paid to single-atom catalysts (SACs) in heterogeneous catalysis because of their unique electronic properties, maximized atomic utilization efficiency, and potential to serve as a bridge between the heterogeneous and homogeneous catalysis. However, SACs can have limited advantages or even constrained applications for the reactions that require designated metallic states with multiple atoms or surface sites with metal-metal bonds. As a cross-dimensional extension to the concept of SACs, fully exposed cluster catalysts (FECCs) offer diverse surface sites formed by an ensemble of metal atoms, for the adsorption and transformation of reactants/intermediates. More importantly, FECCs have the advantage of maximized atom utilization efficiency. Thus, FECCs provide a novel platform to design effective and efficient catalysts for certain chemical processes. This outlook summarizes recent advances and proposes prospective research directions in the design of catalysts and characterizations of FECCs, together with potential challenges.
Funding OrganizationNational Key R&D Program of China ; National Natural Science Foundation of China ; Liaoning Revitalization Talents Program ; Sinopec China ; Tencent Foundation through the XPLORER PRIZE
DOI10.1021/acscentsci.0c01486
Indexed BySCI
Language英语
Funding ProjectNational Key R&D Program of China[2017YFB0602200] ; National Key R&D Program of China[2016YFA0204100] ; National Natural Science Foundation of China[21725301] ; National Natural Science Foundation of China[21821004] ; National Natural Science Foundation of China[91645115] ; National Natural Science Foundation of China[91845201] ; National Natural Science Foundation of China[21961160722] ; Liaoning Revitalization Talents Program[XLYC1907055] ; Sinopec China ; Tencent Foundation through the XPLORER PRIZE
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000624340000009
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:23[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/161805
Collection中国科学院金属研究所
Corresponding AuthorLiu, Hongyang; Ma, Ding
Affiliation1.Peking Univ, Coll Chem & Mol Engn, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China
2.Peking Univ, Coll Engn, Beijing 100871, Peoples R China
3.Peking Univ, BIC ESAT, Beijing 100871, Peoples R China
4.Inner Mongolia Univ, Sch Chem & Chem Engn, Hohhot 010021, Peoples R China
5.Univ New Haven, Chem & Chem Engn Dept, West Haven, CT 06516 USA
6.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
Recommended Citation
GB/T 7714
Peng, Mi,Dong, Chunyang,Gao, Rui,et al. Fully Exposed Cluster Catalyst (FECC): Toward Rich Surface Sites and Full Atom Utilization Efficiency[J]. ACS CENTRAL SCIENCE,2021,7(2):262-273.
APA Peng, Mi,Dong, Chunyang,Gao, Rui,Xiao, Dequan,Liu, Hongyang,&Ma, Ding.(2021).Fully Exposed Cluster Catalyst (FECC): Toward Rich Surface Sites and Full Atom Utilization Efficiency.ACS CENTRAL SCIENCE,7(2),262-273.
MLA Peng, Mi,et al."Fully Exposed Cluster Catalyst (FECC): Toward Rich Surface Sites and Full Atom Utilization Efficiency".ACS CENTRAL SCIENCE 7.2(2021):262-273.
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