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K44合金以及Cr-Ta合金中拓扑密堆相的结构与缺陷的电子显微学研究
其他题名Electron Microscopic Characterization of TCP phase in superalloy K44 and Cr-Ta binary alloy
吴元元
学位类型硕士
导师叶恒强
2007-06-04
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料物理与化学
关键词拓扑密堆相 Σ相 Cr2ta Laves相 Z衬度像
摘要拓扑密堆相是相对于等径原子密堆结构(面心立方、六角密堆)而言的大小不同的原子密堆积的结构,在晶体学中拓扑密堆相由配位数为十二、十四、十五、十六的四类原子密堆而成。具有拓扑密堆结构的金属间化合物的应用非常广泛。但是在高温合金和高合金钢中,拓扑密堆相是脆性相,是需要防止出现的相。自20世纪70年代以来,金属间化合物作为新型功能材料和结构材料得到了广泛深入的研究和发展, 其中Laves相金属间化合物的化学配比是AB2,因其熔点高、高温强度高、高抗氧化能力和高抗蠕变能力而受到高温结构选材的重视。 铸造高温合金K44在长期时效后会析出σ相,通过扫描电镜观察得出在800℃时效10000小时的样品中析出的σ相最多,这些σ相呈细长状均匀的分布在基体中。X射线能谱线扫描分析结果表明σ相富Cr和Co。利用高分辨成像技术,观察到σ相中有两种共生相:H和F相,确定它们与σ相的取向关系。发现σ相中有多种缺陷:不同方向的平移畴界、平移畴界交截和旋转畴,对这些畴界结构进行了系统的分析,通过X射线能谱分析了缺陷处的成分,发现在缺陷处有重元素的富集。 利用真空熔炼炉制备了Cr2Ta的样品,通过XRD分析得出样品都是C14六方结构的Cr2Ta,无C15立方和C36六角结构的衍射峰出现。利用高角环形暗场像技术获得了Cr2Ta的高分辨Z衬度像,直接观察到Ta原子在完整区域和有层错区域的排列构型。通过分析得出该层错属于抽出型层错, 高分辨Z衬度像的分析结果表明该层错是连续堆垛的三层原子的顺序发生反转。
其他摘要The TCP phase is closely packed by different atoms in size, in comparison with the structure which is closely packed by the atoms in same size. In crystallography, four different coordination polyhedrons with coordination numbers 12, 14, 15 and 16 respectively, pack closely to form the TCP phase. Intermetallic compounds with TCP structure have been extensive application these years. But the TCP phases precipitated in superalloy and alloy steel are usually hard 、 brittle and effect the plastic properties of these materials detrimentally, so the formation of TCP phase must be avoided. Since 1970, the intermetallic compounds as new functional materials and structure materials have been deeply investigated. Nowadays the laves phase compounds have been chosen as high temperature structure materials because of their high melting point 、good high temperature intensity 、 high oxidation resistance and creep resistance. SEM observation shows that a large amount of σ phase precipitate from the superalloy K44 aged at 800℃ for 10000h. These σ phases dispersed homogeneously in the matrix with needle-like shape. EDS analysis shows that σ phases enrich more Cr and Co than matrix. From HREM analysis, it is learned that the σ phases have two intergrowth phases: H phase and F phase, and the relationships between them have been determined. Translation domains and rotation domains are found in σ phases and a systemic analysis has been done to these translation domain boundaries and rotation domain boundaries. EDS results show that more heavy elements segregate at the domain boundaries than other areas. The Cr2Ta sample was prepared by vacuum furnace melting. The XRD results show that the structure of sample is C14, and there are no C15 and C36 diffraction apexes detectable. Atomic projection of hexagonal Cr2Ta Laves phase has been directly imaged by Z-contrast imaging at an atomic scale, which provides much more detailed information compared with the conventional coherent high-resolution imaging. Stacking faults with sequence of …stst’st’stst’…are identified, where the three-layer stacks (Ta-Cr-Ta) switch from t to t’ type.
页数70
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17094
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
吴元元. K44合金以及Cr-Ta合金中拓扑密堆相的结构与缺陷的电子显微学研究[D]. 金属研究所. 中国科学院金属研究所,2007.
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