IMR OpenIR
铜的室内加速腐蚀与室外大气腐蚀的相关性研究
其他题名Correlations between Accelerated Laboratory Corrosion Tests and Atmospheric Corrosion Station Tests on Copper
杨敏
学位类型硕士
导师王振尧
2007-06-05
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词 大气腐蚀 相关性 加速实验
摘要本文通过铜在0.01mol/L(NH4)2SO4+0.01mol/LNaHSO3+0.01mol/LNaCl、0.01mol/L (NH4)2SO4 、0.03mol/L(NH4)2SO4三种腐蚀介质中的模拟加速腐蚀实验和沈阳室外大气暴露实验,利用质量损失、腐蚀产物形貌观察及成分分析等方法,研究了铜在室内加速腐蚀和室外大气暴露实验条件下的腐蚀行为,并对所采用的三种加速腐蚀实验方法进行比较,探讨了铜在室内加速腐蚀和室外大气暴露条件大气腐蚀的相关性,由此可以根据室内腐蚀实验的结果预测室外长期暴露的实验结果。 在室内加速腐蚀实验和室外大气暴露实验中,铜的腐蚀失重和实验时间均表现为线性的规律,腐蚀率基本恒定,腐蚀产物没有保护性;对数据进行拟合后,发现铜在该条件下腐蚀失重M(g/m2)与腐蚀时间T(hour)的关系均符合线性规律 M=C+V*T。由室内加速腐蚀实验和室外大气暴露实验的失重结果可以建立两种情况下达到同样的腐蚀失重所需时间的关系式,由此可以通过短期室内加速腐蚀实验推测室外大气暴露实验产生同样腐蚀失重所需要的时间。 在室内加速腐蚀实验和室外大气暴露实验中,铜腐蚀的初期均为局部腐蚀。室外大气暴露实验中和三种加速腐蚀实验中得到的腐蚀产物均主要为CuO、Cu2O及铜的硫酸盐,并且Cu2O的生成贯穿整个腐蚀过程。从腐蚀产物生成的角度来讲,三种加速腐蚀实验方法都可以很好模拟室外大气暴露实验结果。 从模拟性来讲,综合腐蚀形貌、腐蚀产物、表面元素变化三方面考虑,采用混合介质的加速腐蚀实验方法相对差一些,采用较高浓度的单一介质的加速方法效果更好,采用较低浓度的单一介质的加速方法效果次之。 关键词:铜,大气腐蚀,相关性,加速实验
其他摘要ABSTRACT Correlations between Accelerated Laboratory Corrosion Tests and Atmospheric Corrosion Station Tests on Copper Yang Min (Material Science) Supervised by Associate Prof. Wang Zhenyao This work presents results obtained on copper coupons exposed in Shenyang outdoor industrial area. Meanwhile, the results are obtained on copper coupons in accelerated laboratory corrosion tests with three solutions: 0.01mol/L(NH4)2SO4+0.01mol/LNaCl+ 0.01mol/LNaHSO3, 0.01mol/L(NH4)2SO4, 0.03mol/L(NH4)2SO4.The behavior of corrosion of copper in this work was studied through mass loss, surface observation and products analysis. The aim is to identify the corrosion layer composition using several analytical techniques and also to analyze some effects on the corrosion behavior of copper. The correlations between accelerated laboratory corrosion tests and atmospheric corrosion station tests on copper are established allowing the possibility of predicting long-term atmospheric corrosion behavior based on accelerated corrosion tests only. In laboratory tests and Shenyang outdoor test, it is shown that the corrosion process of copper could be described by a formulary of M=C+V*T in which M presents mass loss, and T presents exposure time. It is shown that the corrosion rate of copper is approximately same in the corrosion process and protective properties of copper products are not obtained. In addition, the equation has been established when the same mass loss was reached of copper in outdoor and accelerated tests respectively. This equation could predict exposure time in long-term outdoor tests based on exposure time obtained in accelerated corrosion tests. In laboratory tests and Shenyang outdoor test, local corrosion dominated on surface of copper. The products formed on copper in laboratory tests and Shenyang outdoor test are mainly CuO, Cu2O and copper sulfate, and Cu2O is formed in the whole corrosion process. Considering the corrosion products, corrosion behavior in all accelerated laboratory tests in this work could simulate that in Shenyang outdoor test. Considering the simulation, the accelerated test with mixed solution has the worst simulation, and test with higher concentration solution is better than it with lower concentration solution, evaluated by corrosion morphology, products and elements on corroded surface. Keywords: copper, atmospheric corrosion, correlations, accelerated laboratory tests
页数75
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17095
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
杨敏. 铜的室内加速腐蚀与室外大气腐蚀的相关性研究[D]. 金属研究所. 中国科学院金属研究所,2007.
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