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Weyl Semimetal States Generated Extraordinary Quasi-Linear Magnetoresistance and Nernst Thermoelectric Power Factor in Polycrystalline NbP
Liu, Wei1; Wang, Zhaohui1; Wang, Jinhua2,3; Bai, Hui1; Li, Zhi1; Sun, Jinchang1; Zhou, Xingyuan1; Luo, Jiangfan1; Wang, Wei1; Zhang, Cheng1; Wu, Jinsong1; Sun, Yan4; Zhu, Zengwei2,3; Zhang, Qingjie1; Tang, Xinfeng1
通讯作者Tang, Xinfeng(tangxf@whut.edu.cn)
2022-04-21
发表期刊ADVANCED FUNCTIONAL MATERIALS
ISSN1616-301X
页码10
摘要Unsaturated and extremely large magnetoresistance (MR), as well as the giant Nernst effect, are intriguing transport phenomena in Weyl semimetals, which are technically appealing for potential applications in magneto-electric sensors and transverse thermoelectric conversion. The prominent properties are originated from Weyl semimetal states, i.e., the coexistence of electron and hole pockets combined with linear band dispersion. However, previous studies have been focused on small-sized single crystals, rendering the practical applications of Weyl semimetals. Here, it is reported an unsaturated, quasi-linear MR as well as a very large Nernst power factor PFxy in the prepared centimeter-sized and polycrystalline Weyl semimetal NbP. An extraordinary MR of approximate to 2 x 10(4)% is observed below 60 K with a magnetic field up to 55 T and persists to elevated temperatures. The unusual quasi-linear MR behavior is explained by the theory of classical linear MR arising from structural disorder. The polycrystalline NbP exhibits state-of-the-art PFxy that reaches a maximum value of 74.81 mu W cm(-1) K-2 at 9 T and 220 K, which is 1.5 times larger than its longitudinal thermoelectric power factor PFxx. Given that polycrystalline Weyl semimetal, NbP is suitable for large-scale production, the results pave the way for its practical applications in magneto-electric sensors and transverse thermoelectric conversion.
关键词NbP Nernst thermoelectric power factor polycrystalline quasi-linear magnetoresistance Weyl semimetal states
资助者National Key Research and Development Program of China ; Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities
DOI10.1002/adfm.202202143
收录类别SCI
语种英语
资助项目National Key Research and Development Program of China[2019YFA0704900] ; Natural Science Foundation of China[91963120] ; Natural Science Foundation of China[52150710537] ; Natural Science Foundation of China[12004123] ; Fundamental Research Funds for the Central Universities[WUT: 2021III016GX]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:000789584100001
出版者WILEY-V C H VERLAG GMBH
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/172489
专题中国科学院金属研究所
通讯作者Tang, Xinfeng
作者单位1.Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
2.Huazhong Univ Sci & Technol, Wuhan Natl High Magnet Field Ctr, Wuhan 430074, Peoples R China
3.Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
4.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
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GB/T 7714
Liu, Wei,Wang, Zhaohui,Wang, Jinhua,et al. Weyl Semimetal States Generated Extraordinary Quasi-Linear Magnetoresistance and Nernst Thermoelectric Power Factor in Polycrystalline NbP[J]. ADVANCED FUNCTIONAL MATERIALS,2022:10.
APA Liu, Wei.,Wang, Zhaohui.,Wang, Jinhua.,Bai, Hui.,Li, Zhi.,...&Tang, Xinfeng.(2022).Weyl Semimetal States Generated Extraordinary Quasi-Linear Magnetoresistance and Nernst Thermoelectric Power Factor in Polycrystalline NbP.ADVANCED FUNCTIONAL MATERIALS,10.
MLA Liu, Wei,et al."Weyl Semimetal States Generated Extraordinary Quasi-Linear Magnetoresistance and Nernst Thermoelectric Power Factor in Polycrystalline NbP".ADVANCED FUNCTIONAL MATERIALS (2022):10.
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