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一种高W强化高温合金的组织与性能
其他题名The microstructure and mechanical properties of a superalloy strengthened by high W addition
张艳峰
学位类型硕士
导师孙文儒
2009-05-31
学位授予单位中国科学院金属研究所
学位授予地点金属研究所
学位专业材料学
关键词高温合金 凝固 偏析 热变形 力学性能
摘要本文所研究的是一种高W强化的镍基高温合金,具有很高的热强性,可以在较高的温度下使用。本文系统研究了合金的组织、凝固、均匀化处理、热变形行为和力学性能,以期为该合金的生产和应用提供参考。 研究了合金的铸态组织。合金的组织由γ基体、枝晶间析出的η相和Laves相,以及同时存在于枝晶间和枝晶干的MC和γ′相组成。 利用DSC实验和高温水淬试验研究了合金的凝固行为和凝固偏析。经过分析确定,合金的凝固顺序为:L→γ;L→MC;L→η+Laves。并在凝固结束之后的降温过程中发生γ→η(细针状)和γ→γ′固态反应。在凝固过程中合金各组成元素均表现出不同程度的偏析,其中偏析程度最大的是W、Nb、Ti三种元素。W呈负偏析,Nb、Ti呈正偏析。 通过研究合金中低熔点相的溶解和元素扩散,确定合金的均匀化制度为1150℃×10h+1220℃×40h。经1150℃×10h处理,合金中的低熔点相完全溶入基体,同时合金中析出针状和块状μ相。经1220℃×40h处理,μ相完全溶解,元素偏析基本消除,同时MC碳化物显著溶解变小。 高含量的难熔元素W和其他强化元素的共同作用使合金的热变形困难。利用热模拟试验测试合金在不同组织状态下在不同温度的热加工性能后确认,均匀化态合金和均匀化后μ相呈长针状析出态合金的变形性能较好。据此选择均匀化态作为锻造开坯的原始组织。 铸态合金经均匀化、开坯和热处理得到的组织是基体上均匀分布的颗粒状μ相,尺寸在1μm以下,和圆球形γ′相,尺寸约15μm;晶界上形成连续片状析出相。 合金的拉伸性能和持久性能测试结果表明,合金有较高的室温和高温拉伸强度,这与合金的高W强化和较高程度的γ′相沉淀强化有关。但拉伸塑性随着温度的升高而降低,这是因为晶界没有得到很好的强化。合金在700-750℃具有较好的持久性能,持久样品的断裂以沿晶断裂为主。如果能够改善晶界析出物的分布,合金的高温拉伸塑性和持久性能将得到进一步提高。
其他摘要To improve the stress rupture and creep properties, the element W is added into a superalloy for serving at elevated temperatures. The microstructure at varied state, solidification, homogenization, hot-deformation and properties of the alloy are investigated in this study for the sake of application. The as-cast microstructure of the alloy is made up of γ matrix, η and Laves phases precipitated in the interdendritic region, MC and γ′ phases precipitated at both the dendrite core and interdendritic region. The solidification and segregation of the alloy are studied by DSC and by high-temperature soaking and quenching test. The solidification sequence is determined to be as followings: L→γ; L→MC; L→η+Laves, followed by solid-state reactions of γ→η(needle-like) and γ→γ′. All elements show some extent of segregation, among which the segregation of W, Nb and Ti are greatest. Nb and Ti exhibit normal segregation, while W shows negative segregation. The dissolution of low melting point phases and the diffusion of the elements at high temperature are investigated, and homogenization regime of the alloy is determined to be as followings: 1150℃×10h+1220℃×40h. The low melting point phases are completely dissolved into the γ matrix by the soaking at 1150℃ for10h, while needle-like and massive μ phase particles precipitate during this stage annealing. The μ phase is dissolved and elemental distribution becomes uniform satisfactorily after soaking at 1220℃ for 40h, with the MC carbide dissolving noticeably. The hot deformation of the alloy is difficult due to the high contents of refractory element W and other strengthening elements. Thus the processing abilities of samples with different original microstructures are examined by depressing the samples at varied temperatures with thermal simulation tests. The samples homogenized and homogenized followed by μ needles precipitation soaking have the best hot plasticity. The homogenized structure is selected for forging. The as-cast alloy is homogenized, forged and heat treated. The μ particles with a diameter below 1 μm and globular γ′ particles with a diameter of 15nm are distributed uniformly in the grains of the alloy as heat treated. The plate-like particles are distributed densely along the grain boundary. The tensile and stress rupture properties are tested. The ultimate and yield strength of the alloy at room and elevated temperatures are high, which can be attributed to the solution strengthening of higher W addition and the precipitating strengthening by γ′ phase. But the tensile plasticity decreases with the increasing temperature, because the grain boundaries are not strengthened properly. The alloy has good stress rupture properties at 700℃-750℃. The samples is ruptured with the intergranular fracture mode. The high temperature tensile plasticity and stress rupture property can be ameliorated by the improvement of grain boundary precipitation.
页数81
语种中文
文献类型学位论文
条目标识符http://ir.imr.ac.cn/handle/321006/17268
专题中国科学院金属研究所
推荐引用方式
GB/T 7714
张艳峰. 一种高W强化高温合金的组织与性能[D]. 金属研究所. 中国科学院金属研究所,2009.
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