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Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries
Zhang, Chengzhi1,2; Wang, Fei3; Han, Jian1; Bai, Shuo1; Tan, Jun2; Liu, Jinshui3; Li, Feng1,4
Corresponding AuthorTan, Jun(tanjun@jihualab.com) ; Li, Feng(fli@imr.ac.cn)
2021-06-01
Source PublicationSMALL STRUCTURES
Volume2Issue:6Pages:19
AbstractThe electrode materials are the most critical content for lithium-ion batteries (LIBs) with high energy density for electric vehicles and portable electronics. Considering the high abundance, environmental friendliness, low cost, high capacity, and low operation potential of silicon-based anode, it has been intensively studied as one of the most promising anode materials for high-energy LIBs. However, the widespread application of silicon anode is impeded by the poor electrical conductivity, large volume variation, and unstable solid-electrolyte interfaces films. In the past decade, significant efforts have been demonstrated to tackle these major challenges toward industrial applications. Herein, the focus is on combining with advanced structure like nanostructure and composite with other materials, exploring various new polymer binders, improving electrolyte, different prelithiation strategies, and Si/graphite design to meet commercialization requirements, particularly summarized the progress on areal capacity, initial Coulombic efficiency, and cost. Finally, the guidelines and trends for practical silicon electrodes are presented based on the recent reports.
Keywordanodes energy densities lithium-ion batteries nanostructures silicon
Funding OrganizationNational Natural Science Foundation of China ; National Key R&D Program of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Liaoning Revitalization Talents Program ; Key R&D Plan of Jihua Laboratory
DOI10.1002/sstr.202100009
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51525206] ; National Natural Science Foundation of China[51902316] ; National Key R&D Program of China[2016YFA0200102] ; National Key R&D Program of China[2016YFB0100100] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA22010602] ; Liaoning Revitalization Talents Program[XLYC1908015] ; Key R&D Plan of Jihua Laboratory[X200191TL200]
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000704605100008
PublisherWILEY
Citation statistics
Cited Times:120[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/173063
Collection中国科学院金属研究所
Corresponding AuthorTan, Jun; Li, Feng
Affiliation1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China
2.Ji Hua Lab, Foshan 528000, Guangdong, Peoples R China
3.Hunan Univ, Hunan Prov Key Lab Adv Carbon Mat & Appl Technol, Coll Mat Sci & Engn, Changsha 410082, Peoples R China
4.Shenyang Ind Technol Res Inst Energy Mat & Device, Shenyang, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Chengzhi,Wang, Fei,Han, Jian,et al. Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries[J]. SMALL STRUCTURES,2021,2(6):19.
APA Zhang, Chengzhi.,Wang, Fei.,Han, Jian.,Bai, Shuo.,Tan, Jun.,...&Li, Feng.(2021).Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries.SMALL STRUCTURES,2(6),19.
MLA Zhang, Chengzhi,et al."Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries".SMALL STRUCTURES 2.6(2021):19.
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