Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries

doi:10.1002/sstr.202100009

IMR OpenIR

	Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries
	Zhang, Chengzhi 1,2; Wang, Fei 3; Han, Jian 1; Bai, Shuo 1; Tan, Jun 2; Liu, Jinshui 3; Li, Feng 1,4
通讯作者	Tan, Jun(tanjun@jihualab.com) ; Li, Feng(fli@imr.ac.cn)
	2021-06-01
发表期刊	SMALL STRUCTURES
卷号	2 期号:6 页码:19
摘要	The electrode materials are the most critical content for lithium-ion batteries (LIBs) with high energy density for electric vehicles and portable electronics. Considering the high abundance, environmental friendliness, low cost, high capacity, and low operation potential of silicon-based anode, it has been intensively studied as one of the most promising anode materials for high-energy LIBs. However, the widespread application of silicon anode is impeded by the poor electrical conductivity, large volume variation, and unstable solid-electrolyte interfaces films. In the past decade, significant efforts have been demonstrated to tackle these major challenges toward industrial applications. Herein, the focus is on combining with advanced structure like nanostructure and composite with other materials, exploring various new polymer binders, improving electrolyte, different prelithiation strategies, and Si/graphite design to meet commercialization requirements, particularly summarized the progress on areal capacity, initial Coulombic efficiency, and cost. Finally, the guidelines and trends for practical silicon electrodes are presented based on the recent reports.
关键词	anodes energy densities lithium-ion batteries nanostructures silicon
资助者	National Natural Science Foundation of China ; National Key R&D Program of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Liaoning Revitalization Talents Program ; Key R&D Plan of Jihua Laboratory
DOI	10.1002/sstr.202100009
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51525206] ; National Natural Science Foundation of China[51902316] ; National Key R&D Program of China[2016YFA0200102] ; National Key R&D Program of China[2016YFB0100100] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA22010602] ; Liaoning Revitalization Talents Program[XLYC1908015] ; Key R&D Plan of Jihua Laboratory[X200191TL200]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目	Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000704605100008
出版者	WILEY
引用统计	被引频次：120[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/173063
专题	中国科学院金属研究所
通讯作者	Tan, Jun; Li, Feng
作者单位	1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China 2.Ji Hua Lab, Foshan 528000, Guangdong, Peoples R China 3.Hunan Univ, Hunan Prov Key Lab Adv Carbon Mat & Appl Technol, Coll Mat Sci & Engn, Changsha 410082, Peoples R China 4.Shenyang Ind Technol Res Inst Energy Mat & Device, Shenyang, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Chengzhi,Wang, Fei,Han, Jian,et al. Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries[J]. SMALL STRUCTURES,2021,2(6):19.
APA	Zhang, Chengzhi.,Wang, Fei.,Han, Jian.,Bai, Shuo.,Tan, Jun.,...&Li, Feng.(2021).Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries.SMALL STRUCTURES,2(6),19.
MLA	Zhang, Chengzhi,et al."Challenges and Recent Progress on Silicon-Based Anode Materials for Next-Generation Lithium-Ion Batteries".SMALL STRUCTURES 2.6(2021):19.