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Facile fabrication of graphene encapsulating 3d transition metal nanoparticles as highly active and anti-poisoning catalysts for selective hydrogenation of nitroaromatics
Wu, Genghuang1; Zhao, Linmin2,3; Zong, Mingsheng1; Yu, Peng1; Xie, Jingxin1; Da, Zhijian1; Liu, Hongyang2,3; Rong, Junfeng1
Corresponding AuthorDa, Zhijian(dazhijian.ripp@sinopec.com) ; Liu, Hongyang(liuhy@imr.ac.cn) ; Rong, Junfeng(rongjf.ripp@sinopec.com)
2022-02-15
Source PublicationJOURNAL OF COLLOID AND INTERFACE SCIENCE
ISSN0021-9797
Volume608Pages:1278-1285
AbstractGraphene encapsulating 3d transition metal nanoparticles (Ni, Co, Fe@G) are successfully fabricated through pyrolysis of complexes which are simply prepared via "acid-base reactions" between metal hydroxides and carboxylic acid such as citric acid. In particular, the Ni@G catalyst exhibits outstanding catalytic activity and selectivity (>99%) toward the reduction of various nitroaromatics under mild conditions (1 MPa H-2, 60 degrees C), even in the presence of poisons (CO and thiophene etc.). This "acid-base reactions" based method provides a facile and scalable approach to prepare graphene encapsulating 3d transition metals with wide ranges of applications. (C) 2021 Elsevier Inc. All rights reserved.
KeywordGraphene encapsulation 3d transition metal nanoparticles Chemoselective hydrogenation Anti-poisoning Nitroarenes
Funding OrganizationChina Petrochemical Corporation ; National Key R&D Program of China ; National Natural Science Foundation of China ; Liaoning Revitalization Talents Program ; Dalian National Lab for Clean Energy, (DNL Cooperation Fund)
DOI10.1016/j.jcis.2021.10.105
Indexed BySCI
Language英语
Funding ProjectChina Petrochemical Corporation[420043-4] ; China Petrochemical Corporation[420043-10] ; National Key R&D Program of China[2016YFA0204100] ; National Natural Science Foundation of China[91845201] ; National Natural Science Foundation of China[21961160722] ; National Natural Science Foundation of China[22072162] ; Liaoning Revitalization Talents Program[XLYC1907055] ; Dalian National Lab for Clean Energy, (DNL Cooperation Fund)[202001]
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000744111100007
PublisherACADEMIC PRESS INC ELSEVIER SCIENCE
Citation statistics
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/173627
Collection中国科学院金属研究所
Corresponding AuthorDa, Zhijian; Liu, Hongyang; Rong, Junfeng
Affiliation1.SINOPEC, Res Inst Petr Proc, Beijing 100083, Peoples R China
2.Chinese Acad Sci Inst, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Peoples R China
Recommended Citation
GB/T 7714
Wu, Genghuang,Zhao, Linmin,Zong, Mingsheng,et al. Facile fabrication of graphene encapsulating 3d transition metal nanoparticles as highly active and anti-poisoning catalysts for selective hydrogenation of nitroaromatics[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2022,608:1278-1285.
APA Wu, Genghuang.,Zhao, Linmin.,Zong, Mingsheng.,Yu, Peng.,Xie, Jingxin.,...&Rong, Junfeng.(2022).Facile fabrication of graphene encapsulating 3d transition metal nanoparticles as highly active and anti-poisoning catalysts for selective hydrogenation of nitroaromatics.JOURNAL OF COLLOID AND INTERFACE SCIENCE,608,1278-1285.
MLA Wu, Genghuang,et al."Facile fabrication of graphene encapsulating 3d transition metal nanoparticles as highly active and anti-poisoning catalysts for selective hydrogenation of nitroaromatics".JOURNAL OF COLLOID AND INTERFACE SCIENCE 608(2022):1278-1285.
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