One-Step Growth of Bilayer 2H-1T?MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration

doi:10.1021/acsnano.2c04664

IMR OpenIR

	One-Step Growth of Bilayer 2H-1T?MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration
	Guo, Zenglong 1,2; Wang, Lei 3,4; Han, Mengjiao 5; Zhao, Erding 1,2; Zhu, Liang 1,2; Guo, Weiteng 1,2; Tan, Junyang 6,7; Liu, Bilu 6,7; Chen, Xing-Qiu 3,4; Lin, Junhao 1,2
通讯作者	Liu, Bilu(bilu.liu@sz.tsinghua.edu.cn) ; Chen, Xing-Qiu(xingqiu.chen@imr.ac.cn) ; Lin, Junhao(linjh@sustech.edu.cn)
	2022-07-26
发表期刊	ACS NANO
ISSN	1936-0851
卷号	16 期号:7 页码:11268-11277
摘要	2H???1T??? MoTe2 van der Waals heterostructures (vdWHs) have promising applications in optoelectronics due to a seamlessly homogeneous semiconductor???metal coupled interface. However, the existing methods to fabricate such vdWHs involved complicated steps that may deteriorate the interfacial coupling and are also lacking precise thickness control capability. Here, a one-step growth method was developed to controllably grow bilayer 2H???1T??? MoTe2 vdWHs in the small growth window overlapped for both phases. Atomic-resolution low-voltage transmission electron micros-copy shows the distinct moire?? patterns in the bilayer vdWHs, revealing the epitaxial nature of the top 2H phase with the lattice parameters regulated by the underneath 1T??? phase. Such epitaxially stacked bilayer vdWHs modulate the interlayer coupling by resonating their vibration modes, as unveiled by the angle-resolved polarized Raman spectroscopy and first-principles calculations. Superscript/Subscript Available
关键词	MoTe2 salt-assisted CVD growth van der Waals heterostructure polarized Raman spectroscopy first-principles calculation
资助者	National Natural Science Foundation of China ; Guangdong Innovative and Entrepreneurial Research Team Program ; Shenzhen Science and Technology Program ; Science, Technology and Innovation Commission of Shenzhen Municipality ; Special Funds for the Cultivation of Guangdong College Students Special Funds ; Presidential Fund and Development and Reform Commission of Shenzhen Municipality
DOI	10.1021/acsnano.2c04664
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[11974156] ; National Natural Science Foundation of China[51725103] ; National Natural Science Foundation of China[52188101] ; Guangdong Innovative and Entrepreneurial Research Team Program[2019ZT08C044] ; Shenzhen Science and Technology Program[KQTD20190929173815000] ; Shenzhen Science and Technology Program[20200925161102001] ; Science, Technology and Innovation Commission of Shenzhen Municipality[ZDSYS20190902092905285] ; Special Funds for the Cultivation of Guangdong College Students Special Funds ; Presidential Fund and Development and Reform Commission of Shenzhen Municipality
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目	Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000831245400001
出版者	AMER CHEMICAL SOC
引用统计
文献类型	期刊论文
条目标识符	http://ir.imr.ac.cn/handle/321006/174754
专题	中国科学院金属研究所
通讯作者	Liu, Bilu; Chen, Xing-Qiu; Lin, Junhao
作者单位	1.Southern Univ Sci & Technol, Shenzhen Inst Quantum Sci & Engn SIQSE, Dept Phys, Shenzhen 518055, Peoples R China 2.Southern Univ Sci & Technol, Shenzhen Key Lab Adv Quantum Funct Mat & Devices, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 4.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 5.Songshan Lake Mat Lab, Dongguan 523808, Guangdong, Peoples R China 6.Tsinghua Univ, Shenzhen Geim Graphene Ctr, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China 7.Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China
推荐引用方式 GB/T 7714	Guo, Zenglong,Wang, Lei,Han, Mengjiao,et al. One-Step Growth of Bilayer 2H-1T?MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration[J]. ACS NANO,2022,16(7):11268-11277.
APA	Guo, Zenglong.,Wang, Lei.,Han, Mengjiao.,Zhao, Erding.,Zhu, Liang.,...&Lin, Junhao.(2022).One-Step Growth of Bilayer 2H-1T?MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration.ACS NANO,16(7),11268-11277.
MLA	Guo, Zenglong,et al."One-Step Growth of Bilayer 2H-1T?MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration".ACS NANO 16.7(2022):11268-11277.