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Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O
Li, Z. B.1; Yao, K. L.2,3; Liu, Z. Li2
Corresponding AuthorLi, Z. B.(zongbaoli1982@gmail.com)
2008-06-01
Source PublicationJOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
ISSN0304-8853
Volume320Issue:11Pages:1759-1764
AbstractThe magnetic and thermodynamic properties of the spin-1 tetrahedral "Ni-4'' model have been investigated in terms of the Heisenberg model by algebraic method. It is shown that the Heisenberg model provides an adequate description of the magnetization at low temperatures. The temperature dependence of the specific heat of this model in the vicinity of the midpoint at the rising magnetization M shows remarkable double-peak structure due to the ferromagnetic gapless and anti-ferromagnetic gap excitation of the spin system. The magnetization curve has four clear plateaus, and the susceptibilities exhibit typical anti-ferromagnetic feature, which is well consistent with experimental findings. In particular, the critical magnetic field values H-1 = 5.40 T, H-2 10.69 T, H-3 16.05T and H-4 28.06 T corresponding to the magnetization plateaus are in quantitative agreement with the experimental observations and the former theoretical calculation. (C) 2008 Elsevier B.V. All rights reserved.
Keywordhigh-pulsed magnetic field Heisenberg model magnetization susceptibility
DOI10.1016/j.jmmm.2008.01.033
Indexed BySCI
Language英语
WOS Research AreaMaterials Science ; Physics
WOS SubjectMaterials Science, Multidisciplinary ; Physics, Condensed Matter
WOS IDWOS:000255512200006
PublisherELSEVIER SCIENCE BV
Citation statistics
Cited Times:6[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/93926
Collection中国科学院金属研究所
Corresponding AuthorLi, Z. B.
Affiliation1.Tongren Univ, Dept Phys, Guizhou 554300, Peoples R China
2.Huazhong Univ Sci & Technol, Dept Phys, Wuhan 430074, Peoples R China
3.Chinese Acad Sci, Int Ctr Mat Phys, Shenyang 110016, Peoples R China
Recommended Citation
GB/T 7714
Li, Z. B.,Yao, K. L.,Liu, Z. Li. Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O[J]. JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS,2008,320(11):1759-1764.
APA Li, Z. B.,Yao, K. L.,&Liu, Z. Li.(2008).Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O.JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS,320(11),1759-1764.
MLA Li, Z. B.,et al."Thermodynamic properties of a spin-1 tetrahedron as a model for a molecule-based compound [Mo12O30(mu(2)-OH)(10)H-2{Ni(H2O)(3)}(4)]center dot 14H(2)O".JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 320.11(2008):1759-1764.
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