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Microstructural evolution of [PbZrxTi1-xO3/PbZryTi1-yO3](n) epitaxial multilayers (x/y=0.2/0.4, 0.4/0.6) - dependence on layer thickness
Zhu, Y. L.1; Zheng, S. J.1; Ma, X. L.1; Feigl, L.2; Alexe, M.2; Hesse, D.2; Vrejoiu, I.2
Corresponding AuthorZhu, Y. L.(ylzhu@imr.ac.cn)
2010
Source PublicationPHILOSOPHICAL MAGAZINE
ISSN1478-6435
Volume90Issue:10Pages:1359-1372
AbstractThe microstructure of ferroelectric [PbZrxTi1-xO3/PbZryTi1-yO3](n) epitaxial multilayers (x/y 0.2/0.4, 0.4/0.6) deposited on SrRuO3-coated SrTiO3 substrates by pulsed-laser deposition with different layer periodicity and layer thickness was characterized by means of transmission electron microscopy. Electron diffraction and contrast analysis revealed a very clear and well-separated layer sequence. The microstructures of PbZr0.2Ti0.8O3/PbZr0.4Ti0.6O3 and PbZr0.4Ti0.6O3/PbZr0.6Ti0.4O3 multilayers show a similar tendency in the dependence on the individual layer thickness. Whereas with thick individual layers, tetragonal a-domains are confined to specific layers of the two types of multilayers, below a certain critical thickness of the individual layers, a-domains extend over the whole film. This indicates a transition into a uniform tetragonal lattice and strain state of the whole multilayer. Increasing the layer periodicity further, the interfaces in PbZr0.4Ti0.6O3/PbZr0.6Ti0.4O3 multilayers become rough, and complex a-domain configurations appear.
Keywordferroelectrics transmission electron microscopy microstructure
Funding OrganizationNational Basic Research Program of China ; National Natural Science Foundation of China ; German Research Foundation (DFG)
DOI10.1080/14786430903352656
Indexed BySCI
Language英语
Funding ProjectNational Basic Research Program of China[2009CB623705] ; National Natural Science Foundation of China[50871115] ; German Research Foundation (DFG)[FOR 404] ; German Research Foundation (DFG)[SFB 762]
WOS Research AreaMaterials Science ; Mechanics ; Metallurgy & Metallurgical Engineering ; Physics
WOS SubjectMaterials Science, Multidisciplinary ; Mechanics ; Metallurgy & Metallurgical Engineering ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000276638400008
PublisherTAYLOR & FRANCIS LTD
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.imr.ac.cn/handle/321006/102416
Collection中国科学院金属研究所
Corresponding AuthorZhu, Y. L.
Affiliation1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
2.Max Planck Inst Microstruct Phys, D-06120 Halle, Germany
Recommended Citation
GB/T 7714
Zhu, Y. L.,Zheng, S. J.,Ma, X. L.,et al. Microstructural evolution of [PbZrxTi1-xO3/PbZryTi1-yO3](n) epitaxial multilayers (x/y=0.2/0.4, 0.4/0.6) - dependence on layer thickness[J]. PHILOSOPHICAL MAGAZINE,2010,90(10):1359-1372.
APA Zhu, Y. L..,Zheng, S. J..,Ma, X. L..,Feigl, L..,Alexe, M..,...&Vrejoiu, I..(2010).Microstructural evolution of [PbZrxTi1-xO3/PbZryTi1-yO3](n) epitaxial multilayers (x/y=0.2/0.4, 0.4/0.6) - dependence on layer thickness.PHILOSOPHICAL MAGAZINE,90(10),1359-1372.
MLA Zhu, Y. L.,et al."Microstructural evolution of [PbZrxTi1-xO3/PbZryTi1-yO3](n) epitaxial multilayers (x/y=0.2/0.4, 0.4/0.6) - dependence on layer thickness".PHILOSOPHICAL MAGAZINE 90.10(2010):1359-1372.
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