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Multi-phase heterostructures of flower-like Ni(NiO) decorated on two-dimensional Ti3C2Tx/TiO2 for high-performance microwave absorption properties
Gao, Yang1,2; Du, Heng1; Li, Ruiran3; Zhang, Qipeng1; Fan, Bingbing1,2; Zhao, Biao4; Li, Ning1; Wang, Xiaohui5; Chen, Yongqiang1; Zhang, Rui1,4
通讯作者Fan, Bingbing(fanbingbing@zzu.edu.cn) ; Zhao, Biao(biao_zhao@zua.edu.cn)
2021-04-15
发表期刊CERAMICS INTERNATIONAL
ISSN0272-8842
卷号47期号:8页码:10764-10772
摘要Three-dimensional flower-like Ni(NiO) decorated on two-dimensional Ti3C2Tx/TiO2 composites were successfully synthesized by an in situ solvothermal reaction, and the electromagnetic (EM) wave absorption performance of the hybrids were explored at 2.00-18.00 GHz. The as-prepared Ni(NiO)/Ti3C2Tx/TiO2 composites include flower-like Ni(NiO) with uniform distribution on the surface of Ti3C2Tx MXenes and part of them get into the space between interlayers. The Ni(NiO)/Ti3C2Tx/TiO2 composites exhibit a maximum reflection loss (RL) value of 41.74 dB at 14.96 GHz with the absorber thickness of merely 1.3 mm and the effective absorption bandwidth (EAB) reaches 3.20 GHz. The outstanding electromagnetic wave absorbing performance can be attributed to the dielectric loss of Ti3C2Tx MXenes and multi-phase heterostructures, the magnetic loss of Ni(NiO) and their synergistic loss mechanism. Moreover, the zigzag path formed by flower-like Ni(NiO) also has a great consumption effect on electromagnetic waves by incurring the eddy current under the affect of alternating EM waves. The laminated structure of Ti3C2Tx MXenes also dissipates microwaves by offering the space for multiple reflections and scattering. This paper furnished a novel modus for synthesizing original EM wave absorption materials and making the balance among thickness, broad bandwidth, oxidation resistance and light weight, which makes Ni(NiO)/Ti3C2Tx/TiO2 composites a hopeful material for microwave absorption (MA).
关键词Ni(NiO)/Ti3C2Tx/TiO2 composites Multi-phase heterostructures Dielectric loss Microwave absorption
资助者National Natural Science Foundation of China (NSFC) ; Natural Science Research Project of Henan Educational Committee
DOI10.1016/j.ceramint.2020.12.193
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China (NSFC)[U2004177] ; National Natural Science Foundation of China (NSFC)[51802289] ; Natural Science Research Project of Henan Educational Committee[20A430001]
WOS研究方向Materials Science
WOS类目Materials Science, Ceramics
WOS记录号WOS:000631956700001
出版者ELSEVIER SCI LTD
引用统计
被引频次:26[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.imr.ac.cn/handle/321006/162202
专题中国科学院金属研究所
通讯作者Fan, Bingbing; Zhao, Biao
作者单位1.Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450001, Peoples R China
2.Anhui Normal Univ, Minist Educ, Key Lab Funct Mol Solids, Wuhu 241000, Peoples R China
3.Zhengzhou Univ, Sch Civil Engn, Zhengzhou 450001, Peoples R China
4.Zhengzhou Univ Aeronaut, Sch Mat Sci & Engn, Henan Key Lab Aeronaut Mat & Applicat Technol, Zhengzhou 450046, Peoples R China
5.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
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GB/T 7714
Gao, Yang,Du, Heng,Li, Ruiran,et al. Multi-phase heterostructures of flower-like Ni(NiO) decorated on two-dimensional Ti3C2Tx/TiO2 for high-performance microwave absorption properties[J]. CERAMICS INTERNATIONAL,2021,47(8):10764-10772.
APA Gao, Yang.,Du, Heng.,Li, Ruiran.,Zhang, Qipeng.,Fan, Bingbing.,...&Zhang, Rui.(2021).Multi-phase heterostructures of flower-like Ni(NiO) decorated on two-dimensional Ti3C2Tx/TiO2 for high-performance microwave absorption properties.CERAMICS INTERNATIONAL,47(8),10764-10772.
MLA Gao, Yang,et al."Multi-phase heterostructures of flower-like Ni(NiO) decorated on two-dimensional Ti3C2Tx/TiO2 for high-performance microwave absorption properties".CERAMICS INTERNATIONAL 47.8(2021):10764-10772.
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